中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
New selection rule of resonant Raman scattering in MoS2 monolayer under circular polarization

文献类型:期刊论文

作者Huang, Jianqi1,2; Liu, Zhiyong1,2; Yang, Teng1,2; Zhang, Zhidong1,2
刊名JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
出版日期2022-03-10
卷号102页码:132-136
关键词First principles calculation Resonant Raman Helicity selection rule MoS2 monolayer
ISSN号1005-0302
DOI10.1016/j.jmst.2021.05.080
通讯作者Yang, Teng(yangteng@imr.ac.cn)
英文摘要The first-order resonant Raman spectra of monolayer MoS2 are calculated under the circularly polarized photoexcitation. The anomalously nonzero Raman intensity of the in-plane E mode under the (Z) over bar(sigma(+)sigma(+))Z or (Z) over bar(sigma(-)sigma(-))Z geometry, which goes against the conventional selection rule, appears under some circum- stances when optical absorption occurs at some special reciprocal points between the zone-center Gamma and the zone-edge-center M points. At that moment, the valley selectivity to the circular polarization is lifted. The analysis shows that the anomalous Raman intensity of the E mode for the same circularly polarized incident and scattered light is consistent with the pseudo-angular-momentum conservation law. The calculated E Raman tensor of monolayer MoS2 is found to vary with laser energy. The two diagonal terms of the Raman tensor change their signs from mutually opposite to the same when the relative intensity of the in-plane E mode to the out-of-plane A(1)' mode increases, indicating the increasingly important role played by the Frolich-type electron-phonon interaction over the deformation potential. Our study may shed new light on the understanding of the novel electron-photon process and assist in the design of new type of optoelectronic devices. (C) 2022 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology.
资助项目National Natural Sci-ence Foundation of China[52031014] ; National Natural Sci-ence Foundation of China[51702146] ; National Key R&D Program of China[2017YFA0206301]
WOS研究方向Materials Science ; Metallurgy & Metallurgical Engineering
语种英语
WOS记录号WOS:000778396100007
出版者JOURNAL MATER SCI TECHNOL
资助机构National Natural Sci-ence Foundation of China ; National Key R&D Program of China
源URL[http://ir.imr.ac.cn/handle/321006/172933]  
专题金属研究所_中国科学院金属研究所
通讯作者Yang, Teng
作者单位1.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
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Huang, Jianqi,Liu, Zhiyong,Yang, Teng,et al. New selection rule of resonant Raman scattering in MoS2 monolayer under circular polarization[J]. JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,2022,102:132-136.
APA Huang, Jianqi,Liu, Zhiyong,Yang, Teng,&Zhang, Zhidong.(2022).New selection rule of resonant Raman scattering in MoS2 monolayer under circular polarization.JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,102,132-136.
MLA Huang, Jianqi,et al."New selection rule of resonant Raman scattering in MoS2 monolayer under circular polarization".JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY 102(2022):132-136.

入库方式: OAI收割

来源:金属研究所

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