中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Flux-Closure Domains in PbTiO3/SrTiO3 Multilayers Mediated without Tensile Strain

文献类型:期刊论文

作者Zhang, Si-Rui2; Zhu, Mei-Xiong1,3; Suriyaprakash, Jagadeesh4; Liu, Jin-Mei2; Du, Tao2; Wang, Yu-Jia1; Long, Chang-Bai5; Liao, Min2
刊名JOURNAL OF PHYSICAL CHEMISTRY C
出版日期2022-03-10
卷号126期号:9页码:4630-4637
ISSN号1932-7447
DOI10.1021/acs.jpcc.1c10057
通讯作者Long, Chang-Bai(longchangbai@126.com) ; Liao, Min(mliao@xidian.edu.cn)
英文摘要Ferroelectric flux-closure domains are promising for carrying information with ultrahigh-density capacities. Particularly, epitaxial tensile strains from external substrates are believed to be important for the formation of these flux-closure domains, but they may limit corresponding applications as high-density memory units. Herein, via pulsed laser deposition method, PbTiO3/SrTiO3 multilayered films are deposited on the cubic (001)-oriented SrTiO3 substrate, which is barely a misfit strain with a PbTiO3 film. The interaction between 90 degrees domains and insulation boundaries in PbTiO3 layers forms the three different flux-closure domains in the multilayered film structure without tensile strain. The complex flux-closure domain structure is investigated by advanced transmission electron microscopy, which is determined to be the width of the a1(1) and a1(2) domains, and the width of the a domains is subject to the thickness of the bottom PbTiO3 layer. Because the bottom PbTiO3 film thickness is proportional to the width and distance between the a1(1) and a1(2) domains, we can easily obtain various flux-closure domain configurations by varying the bottom and top PbTiO3 film thickness ratios. Furthermore, the creation of the flux-closure domain in PbTiO3 films is corroborated by the phenomenological theory. This finding allows us to manipulate domains in order to create and construct novel nanoscale ferroelectric devices with exotic properties.
资助项目National Natural Science Foundation of China[51901166] ; National Natural Science Foundation of China[52072324] ; National Natural Science Foundation of China[52122101] ; Fundamental Research Funds for the Central Universities[JB191404] ; Youth Innovation Promotion Association CAS[2021187]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
语种英语
WOS记录号WOS:000772201900036
出版者AMER CHEMICAL SOC
资助机构National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Youth Innovation Promotion Association CAS
源URL[http://ir.imr.ac.cn/handle/321006/173016]  
专题金属研究所_中国科学院金属研究所
通讯作者Long, Chang-Bai; Liao, Min
作者单位1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
2.Xidian Univ, Sch Adv Mat & Nanotechnol, Xian 710071, Peoples R China
3.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China
4.South China Normal Univ, Sch Informat & Optoelect Sci & Engn, Guangdong Prov Key Lab Nanophoton Funct Mat & Dev, Guangzhou 510006, Peoples R China
5.Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Si-Rui,Zhu, Mei-Xiong,Suriyaprakash, Jagadeesh,et al. Flux-Closure Domains in PbTiO3/SrTiO3 Multilayers Mediated without Tensile Strain[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2022,126(9):4630-4637.
APA Zhang, Si-Rui.,Zhu, Mei-Xiong.,Suriyaprakash, Jagadeesh.,Liu, Jin-Mei.,Du, Tao.,...&Liao, Min.(2022).Flux-Closure Domains in PbTiO3/SrTiO3 Multilayers Mediated without Tensile Strain.JOURNAL OF PHYSICAL CHEMISTRY C,126(9),4630-4637.
MLA Zhang, Si-Rui,et al."Flux-Closure Domains in PbTiO3/SrTiO3 Multilayers Mediated without Tensile Strain".JOURNAL OF PHYSICAL CHEMISTRY C 126.9(2022):4630-4637.

入库方式: OAI收割

来源:金属研究所

浏览0
下载0
收藏0
其他版本

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。