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Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries

文献类型：期刊论文

作者Zhang, Chengzhi2,3; Wang, Fei4; Han, Jian2; Bai, Shuo2; Tan, Jun3; Liu, Jinshui4; Li, Feng1,2
刊名SMALL STRUCTURES
出版日期2021-06-01
卷号2期号:6页码:19
关键词anodes energy densities lithium-ion batteries nanostructures silicon
DOI10.1002/sstr.202100009
通讯作者Tan, Jun(tanjun@jihualab.com) ; Li, Feng(fli@imr.ac.cn)
英文摘要The electrode materials are the most critical content for lithium-ion batteries (LIBs) with high energy density for electric vehicles and portable electronics. Considering the high abundance, environmental friendliness, low cost, high capacity, and low operation potential of silicon-based anode, it has been intensively studied as one of the most promising anode materials for high-energy LIBs. However, the widespread application of silicon anode is impeded by the poor electrical conductivity, large volume variation, and unstable solid-electrolyte interfaces films. In the past decade, significant efforts have been demonstrated to tackle these major challenges toward industrial applications. Herein, the focus is on combining with advanced structure like nanostructure and composite with other materials, exploring various new polymer binders, improving electrolyte, different prelithiation strategies, and Si/graphite design to meet commercialization requirements, particularly summarized the progress on areal capacity, initial Coulombic efficiency, and cost. Finally, the guidelines and trends for practical silicon electrodes are presented based on the recent reports.
资助项目National Natural Science Foundation of China[51525206] ; National Natural Science Foundation of China[51902316] ; National Key R&D Program of China[2016YFA0200102] ; National Key R&D Program of China[2016YFB0100100] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA22010602] ; Liaoning Revitalization Talents Program[XLYC1908015] ; Key R&D Plan of Jihua Laboratory[X200191TL200]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
语种英语
WOS记录号WOS:000704605100008
出版者WILEY
资助机构National Natural Science Foundation of China ; National Key R&D Program of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Liaoning Revitalization Talents Program ; Key R&D Plan of Jihua Laboratory
源URL[http://ir.imr.ac.cn/handle/321006/173062]  
专题金属研究所_中国科学院金属研究所
通讯作者Tan, Jun; Li, Feng
作者单位1.Shenyang Ind Technol Res Inst Energy Mat & Device, Shenyang, Peoples R China
2.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China
3.Ji Hua Lab, Foshan 528000, Guangdong, Peoples R China
4.Hunan Univ, Hunan Prov Key Lab Adv Carbon Mat & Appl Technol, Coll Mat Sci & Engn, Changsha 410082, Peoples R China
推荐引用方式
GB/T 7714		 Zhang, Chengzhi,Wang, Fei,Han, Jian,et al. Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries[J]. SMALL STRUCTURES,2021,2(6):19.
APA Zhang, Chengzhi.,Wang, Fei.,Han, Jian.,Bai, Shuo.,Tan, Jun.,...&Li, Feng.(2021).Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries.SMALL STRUCTURES,2(6),19.
MLA Zhang, Chengzhi,et al."Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries".SMALL STRUCTURES 2.6(2021):19.

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来源：金属研究所

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