Experimental Insights Into the In Situ Formation and Dissociation of Gas Hydrate in Sediments of Shenhu, South China Sea
文献类型：期刊论文
| 作者 | Zhang, Qian3,4,7; Qin, Xuwen5,6; Zhang, Hong3,4,7; Dong, Yanhui3,4,7; Lu, Cheng2,5,6; Li, Shouding3,4,7; Xiao, Luokun3,4,7; Ma, Chao5,6; Bian, Hang1,2 |
| 刊名 | FRONTIERS IN EARTH SCIENCE
 |
| 出版日期 | 2022-05-11 |
| 卷号 | 10页码:10 |
| 关键词 | gas hydrate sediment formation and dissociation nuclear magnetic resonance pore habit |
| DOI | 10.3389/feart.2022.882701 |
| 英文摘要 | Natural gas hydrates as sustainable energy resources are inherently affected by mineral surfaces and confined spaces in reservoirs. However, the habits of hydrates in geological sediments are still an open question. In this work, we systemically studied the process of hydrate formation and dissociation in sediments from the Shenhu area of the South China Sea to examine the evolution of hydrate saturation and permeability in sediments and their relationship. Characterization of samples indicates that sediments of the Shenhu area are mainly composed of clay and fine sand grains and provide a large number of nanopores for hydrate accumulation. For in situ observations enabled by low-field nuclear magnetic resonance methods, the formation of hydrates shows a different kinetic behavior with an induction time compared to hydrate dissociation. Estimated by variations of hydrate saturation (%) over time, the rate of hydrate formation is around 12%/min, while the dissociation rate increases to 3%/min with the higher temperature. With the presence of hydrates, pore space and thus permeability of sediments decreased obviously by one and three orders of magnitude when the hydrate saturation is 20 and 45%, respectively. Compared to models with the assumption of grain-coating and pore-filling hydrates, the tendency of permeability evolution from NMR measurements is between fitted lines from models. It highlights that the existing models considering a single pattern of hydrate growth cannot precisely describe the relationship between permeability and hydrate saturation. Hybrid hydrate habits coexist in sediments resulting from heterogeneous pore structures and thus complex gas-water distributions. |
| WOS关键词 | PERMEABILITY ; SAND ; SATURATION ; PARTICLE ; SIZES ; AREA |
| WOS研究方向 | Geology |
| 语种 | 英语 |
| 出版者 | FRONTIERS MEDIA SA |
| WOS记录号 | WOS:000802277800001 |
| 源URL | [http://ir.iggcas.ac.cn/handle/132A11/105989]  |
| 专题 | 地质与地球物理研究所_中国科学院页岩气与地质工程重点实验室 |
| 通讯作者 | Dong, Yanhui |
| 作者单位 | 1.China Univ Geosci, Sch Energy Resources, Beijing, Peoples R China 2.China Geol Survey, Ctr Oil & Nat Gas Resource Explorat, Beijing, Peoples R China 3.Univ Chinese Acad Sci, Beijing, Peoples R China 4.Chinese Acad Sci, Inst Geol & Geophys, Key Lab Shale Gas & Geoengn, Beijing, Peoples R China 5.Natl Engn Res Ctr Gas Hydrate Explorat & Dev, Guangzhou, Peoples R China 6.China Geol Survey, Guangzhou Marine Geol Survey, Guangzhou, Peoples R China 7.Chinese Acad Sci, Innovat Acad Earth Sci, Beijing, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Qian,Qin, Xuwen,Zhang, Hong,et al. Experimental Insights Into the In Situ Formation and Dissociation of Gas Hydrate in Sediments of Shenhu, South China Sea[J]. FRONTIERS IN EARTH SCIENCE,2022,10:10. |
| APA | Zhang, Qian.,Qin, Xuwen.,Zhang, Hong.,Dong, Yanhui.,Lu, Cheng.,...&Bian, Hang.(2022).Experimental Insights Into the In Situ Formation and Dissociation of Gas Hydrate in Sediments of Shenhu, South China Sea.FRONTIERS IN EARTH SCIENCE,10,10. |
| MLA | Zhang, Qian,et al."Experimental Insights Into the In Situ Formation and Dissociation of Gas Hydrate in Sediments of Shenhu, South China Sea".FRONTIERS IN EARTH SCIENCE 10(2022):10. |
入库方式： OAI收割
来源：地质与地球物理研究所
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