Facile fabrication of self-healing silicone-based poly(urea-thiourea)/tannic acid composite for anti-biofouling
文献类型：期刊论文
| 作者 | Sun, Jiawen1,2,4,5; Liu, Chao1,3; Duan, Jizhou1,2,4,5 ; Liu, Jie5; Dong, Xucheng1,2,4,5; Zhang, Yimeng1,2,5; Wang, Ning1,2,4,5; Wang, Jing1,2,4,5; Hou, Baorong1,2,4,5
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| 刊名 | JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
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| 出版日期 | 2022-10-10 |
| 卷号 | 124页码:1-13 |
| 关键词 | Poly(dimethylsiloxane) Poly(urea-thiourea) Self-healing Hydrogen bonding Marine antifouling Tannic acid |
| ISSN号 | 1005-0302 |
| DOI | 10.1016/j.jmst.2022.01.026 |
| 通讯作者 | Duan, Jizhou(duanjz@qdio.ac.cn) |
| 英文摘要 | A novel silicone-based poly(urea-thiourea)/tannic acid composite (PDMS-P(Ua-TUa)-TA) with excellent mechanical, self-healing and antifouling properties is developed. The multiple dynamic hydrogen bonds formed by thiourea groups, urea groups, and tannic acid (TA) molecules ensured a tough elastomer (ultimate strength: 2.47 MPa) with high stretchability (-10 0 0%). TA molecules as partial hydrogen bonding cross-linking sites interacted rapidly with urea and thiourea groups before the migration of polymer chains, resulting in fast and efficient self-healing. Scratches on the film completely disappeared within 12 min, and the repair efficiency of strength was up to 98.4% within 3 h under ambient condition. Self healing behavior was also evaluated in artificial seawater and the healing efficiency (HE) was 95.1%. Furthermore, TA uniformly dispersed in the polymer matrix provides good antibacterial and anti-diatom properties, as well as strong adhesion to the substrate (-2.2 MPa). Laboratory bioassays against marine bacteria adhesion (-96%,-95% and-93% reduction for P. sp., E. coli, and S. aureus, respectively) and diatom attachment (-84% reduction) demonstrated an outstanding antifouling property of the PDMSP(Ua-TUa)-TA. This work provides a promising pathway towards the development of high-performance silicone-based coatings for marine anti-biofouling. (c) 2022 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology. |
| 资助项目 | Basic Frontier Science Research Program of Chinese Academy of Sciences[ZDBS-LY-DQC025] ; National Natural Science Foundation of China[41706080] ; Shandong Key Laboratory of Corrosion Science |
| WOS研究方向 | Materials Science ; Metallurgy & Metallurgical Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000788133600001 |
| 出版者 | JOURNAL MATER SCI TECHNOL |
| 源URL | [http://ir.qdio.ac.cn/handle/337002/178912]  |
| 专题 | 海洋研究所_海洋腐蚀与防护研究发展中心 |
| 通讯作者 | Duan, Jizhou |
| 作者单位 | 1.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China 2.Chinese Acad Sci, Ctr Ocean Megasci, Qingdao 266071, Peoples R China 3.Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100039, Peoples R China 5.Pilot Natl Lab Marine Sci & Technol Qingdao, Open Studio Marine Corros & Protect, Qingdao 266237, Peoples R China |
| 推荐引用方式 GB/T 7714 | Sun, Jiawen,Liu, Chao,Duan, Jizhou,et al. Facile fabrication of self-healing silicone-based poly(urea-thiourea)/tannic acid composite for anti-biofouling[J]. JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,2022,124:1-13. |
| APA | Sun, Jiawen.,Liu, Chao.,Duan, Jizhou.,Liu, Jie.,Dong, Xucheng.,...&Hou, Baorong.(2022).Facile fabrication of self-healing silicone-based poly(urea-thiourea)/tannic acid composite for anti-biofouling.JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,124,1-13. |
| MLA | Sun, Jiawen,et al."Facile fabrication of self-healing silicone-based poly(urea-thiourea)/tannic acid composite for anti-biofouling".JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY 124(2022):1-13. |
入库方式： OAI收割
来源：海洋研究所
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