Oxygen vacancy tuned oxidase mimic through selenium-doping ultrathin 2D Ni-V mixed metal oxide and antibacterial application
文献类型：期刊论文
| 作者 | Chen, Chao1,2 ; Wang, Yi1,2; Zhang, Dun1,2
|
| 刊名 | JOURNAL OF ALLOYS AND COMPOUNDS
 |
| 出版日期 | 2022-09-15 |
| 卷号 | 915页码:10 |
| 关键词 | Mixed metal oxide Nanosheet Enzyme mimic Doping Antibacterial |
| ISSN号 | 0925-8388 |
| DOI | 10.1016/j.jallcom.2022.165446 |
| 通讯作者 | Wang, Yi(wangyi@qdio.ac.cn) ; Zhang, Dun(zhangdun@qdio.ac.cn) |
| 英文摘要 | To develop effective and low-cost enzyme-like nanomaterials in the antibacterial field, we designed an easily performed and highly specific approach to obtain novel ultrathin Ni-V mixed metal oxides (MMOs) with rich oxygen vacancy. Herein, a selenium (Se) doped novel ultrathin Ni-V MMOs were derived from Ni-V layered double hydroxide (LDHs) with Se powder in N-2 instead of direct calcination in the air successfully. After Se doped, the acquired Ni-V MMOs exhibited richer oxygen vacancy and more changeable elemental state, which can drastically promote the oxidase (OXD)/peroxidase (POD)-like activity increasing nearly 2 times compared with Ni-V MMOs. Se-doping endow 3NiV-Se-350 the unique 2D hierarchical nanostructure and the richest oxygen vacancy. More interesting, Se doped Ni-V MMOs calcinated at 350 ? with a Ni/V molar ratio of 3:1 show the best OXD/POD mimic activity among different Ni/V molar ratios, and possess a good reusability for 7 cycles. Mimic activity of 3NiV-Se-350 was attributed to the reactive oxygen species (ROS), such as center dot OH and center dot O-2(-). 3NiV-Se-350 also exhibit bactericidal rate of 71.04% without H2O2 and 98.89% in the presence of H2O2 against E. coli through generating center dot O-2(-). (C) 2022 Elsevier B.V. All rights reserved. |
| 资助项目 | National Natural Science Foundation of China[41776090] ; National Natural Science Foundation of China[41976032] ; China Postdoctoral Science Foundation[2020M682244] ; China Postdoctoral Science Foundation[2021T140673] |
| WOS研究方向 | Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000807109000001 |
| 出版者 | ELSEVIER SCIENCE SA |
| 源URL | [http://ir.qdio.ac.cn/handle/337002/179497]  |
| 专题 | 海洋研究所_海洋腐蚀与防护研究发展中心 |
| 通讯作者 | Wang, Yi; Zhang, Dun |
| 作者单位 | 1.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China 2.Pilot Natl Lab Marine Sci & Technol Qingdao, Open Studio Marine Corros & Protect, 1 Wenhai Rd, Qingdao 266237, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Chao,Wang, Yi,Zhang, Dun. Oxygen vacancy tuned oxidase mimic through selenium-doping ultrathin 2D Ni-V mixed metal oxide and antibacterial application[J]. JOURNAL OF ALLOYS AND COMPOUNDS,2022,915:10. |
| APA | Chen, Chao,Wang, Yi,&Zhang, Dun.(2022).Oxygen vacancy tuned oxidase mimic through selenium-doping ultrathin 2D Ni-V mixed metal oxide and antibacterial application.JOURNAL OF ALLOYS AND COMPOUNDS,915,10. |
| MLA | Chen, Chao,et al."Oxygen vacancy tuned oxidase mimic through selenium-doping ultrathin 2D Ni-V mixed metal oxide and antibacterial application".JOURNAL OF ALLOYS AND COMPOUNDS 915(2022):10. |
入库方式： OAI收割
来源：海洋研究所
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