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Determination of anionic perfluorinated compounds in water samples using cationic fluorinated metal organic framework membrane coupled with UHPLC-MS/MS

文献类型：期刊论文

作者Li, Shuang1; Ma, Jiping1; Wu, Gege1; Li, Jinhua2,3,6; Ostovan, Abbas2,3,6; Song, Zhihua4; Wang, Xiaoyan5; Chen, Lingxin2,3,6
刊名JOURNAL OF HAZARDOUS MATERIALS
出版日期2022-05-05
卷号429页码:11
关键词Cationic metal organic frameworks (iMOFs) Mixed-matrix membrane (MMM) Dispersion membrane extraction (DME) Perfluorinated compounds (PFCs) Ultra-high performance liquid chromatography-tandem mass spectrometry (UHPLC-MS MS)
ISSN号0304-3894
DOI10.1016/j.jhazmat.2022.128333
通讯作者Ma, Jiping(majiping2012@163.com) ; Chen, Lingxin(lxchen@yic.ac.cn)
英文摘要Global concerns stem from the environmental crisis have compelled researchers to develop selective and sensitive methods for the identification and measurement of emerging pollutants in the environmental matrices. The cationic F-TMU-66+Cl-/polyvinylidene fluoride metal-organic frameworks (MOFs) mixed matrix membrane (FTMU-66+Cl-/PVDF MMM) was synthesized and used as a versatile adsorbent with multiple binding sites for the simultaneous extraction of twelve anionic perfluorinated compounds (PFCs) from reservoir water samples. The physical and chemical characteristics of the materials, as well as adsorption mechanism were fully surveyed by various instrumental techniques. Important extraction parameters, including amount of MOFs, pH, desorption conditions, and salinity were systematically investigated and optimized. The combination of dispersive membrane solid extraction based on F-TMU-66+Cl-/PVDF MMM with ultra-high performance liquid chromatography tandem mass spectrometry provided ultra-low limit of detections within the range of 0.03-0.48 ng/L. By virtue of the simplicity and robustness of the extraction procedure, high sensitivity of detection scheme, good stability and selectivity of the F-TMU-66+Cl-/PVDF MMM, the developed method exhibits excellent practicability for ultra trace analysis of anionic PFCs in water samples.
WOS关键词SELECTIVE ADSORPTION ; REMOVAL ; SUBSTANCES ; SEPARATION ; ADSORBENT ; TOXICITY ; CAPACITY ; BINDING ; MATRIX
WOS研究方向Engineering ; Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000752488700002
资助机构National Natural Science Foundation of China ; Natural Science Foundation of Shandong Province of China ; Science and Technology Innovation Development Plan of Yantai City of China ; Chinese Academy of Sciences President's International Fellowship Initiative ; Taishan Scholar Project Special Funding
源URL[http://ir.yic.ac.cn/handle/133337/31489]  
专题烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
烟台海岸带研究所_山东省海岸带环境工程技术研究中心
通讯作者Ma, Jiping; Chen, Lingxin
作者单位1.Qingdao Univ Technol, Sch Environm & Municipal Engn, Qingdao 266033, Peoples R China
2.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn & Technol, Yantai 264003, Peoples R China
3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
4.Yantai Univ, Minist Educ, Key Lab Mol Pharmacol & Drug Evaluat,Sch Pharm, Collaborat Innovat Ctr Adv Drug Delivery Syst & B, Yantai 264005, Peoples R China
5.Binzhou Med Univ, Sch Pharm, Yantai 264003, Peoples R China
6.Chinese Acad Sci, Ctr Ocean Megasci, Qingdao 266071, Peoples R China
推荐引用方式
GB/T 7714		 Li, Shuang,Ma, Jiping,Wu, Gege,et al. Determination of anionic perfluorinated compounds in water samples using cationic fluorinated metal organic framework membrane coupled with UHPLC-MS/MS[J]. JOURNAL OF HAZARDOUS MATERIALS,2022,429:11.
APA Li, Shuang.,Ma, Jiping.,Wu, Gege.,Li, Jinhua.,Ostovan, Abbas.,...&Chen, Lingxin.(2022).Determination of anionic perfluorinated compounds in water samples using cationic fluorinated metal organic framework membrane coupled with UHPLC-MS/MS.JOURNAL OF HAZARDOUS MATERIALS,429,11.
MLA Li, Shuang,et al."Determination of anionic perfluorinated compounds in water samples using cationic fluorinated metal organic framework membrane coupled with UHPLC-MS/MS".JOURNAL OF HAZARDOUS MATERIALS 429(2022):11.

入库方式： OAI收割

来源：烟台海岸带研究所

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