Vinylene Flanked Naphtho[1,2-c:5,6-c ']bis[1,2,5]thiadiazole Polymer for Low-Crystallinity Ambipolar Transistors
文献类型：期刊论文
| 作者 | Liang, Xianfeng1,2; Chen, Yanlin1; Jiao, Xuechen3; Heeney, Martin4,5; McNeill, Christopher R.3; Dong, Lichun1; Zhou, Cailong1; Liu, Zitong6; Tan, Luxi1 |
| 刊名 | MACROMOLECULES
 |
| 出版日期 | 2022-01-11 |
| 卷号 | 55期号:1页码:331-337 |
| ISSN号 | 0024-9297 |
| DOI | 10.1021/acs.macromol.1c02253 |
| 通讯作者 | Heeney, Martin(m.heeney@imperial.ac.uk) ; Liu, Zitong(zitong_@iccas.ac.cn) ; Tan, Luxi(tanluxi@cqu.edu.cn) |
| 英文摘要 | High charge carrier mobility in organic semiconductors is usually accomplished by its high crystallinity, yet, which, often leads to poor mechanical resilience, limiting their performance in flexible devices. In this work, a naphtho[1,2-c:5,6c']bi-s[1,2,5]thiadiazole (NT)-based polymer PNztDTV containing multiple vinyl linkages was reported, exhibiting excellent ambipolar OFET performance, with hole and electron mobility up to 1.0 (mu(h)) and 0.4 (mu(e)) cm(2) V-1 s(-1), respectively. The GIWAXS analysis revealed overall a rather weak crystallinity in its thin film, yet with considerably strong localized pi-pi intermolecular interaction. The simultaneous low crystallinity and high performance of PNztDTV imply promising potential in flexible electronics, which is presumably resulted by the isomerization of the vinylene linkage and pi-expanded NT core. |
| 资助项目 | China Scholarship Council ; National Natural Science Foundation of China[NSFC 21404107] ; Chongqing Science & Technology Commission[cstc2018jcyjAX0091] ; EPSRC[EP/T028513/1] |
| WOS研究方向 | Polymer Science |
| 语种 | 英语 |
| WOS记录号 | WOS:000766223400032 |
| 出版者 | AMER CHEMICAL SOC |
| 源URL | [http://119.78.100.138/handle/2HOD01W0/15021]  |
| 专题 | 中国科学院重庆绿色智能技术研究院 |
| 通讯作者 | Heeney, Martin; Liu, Zitong; Tan, Luxi |
| 作者单位 | 1.Chongqing Univ, Sch Chem & Chem Engn, Chongqing 401331, Peoples R China 2.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China 3.Monash Univ, Dept Mat Sci & Engn, Clayton, Vic 3800, Australia 4.Imperial Coll London, Dept Chem, London W12 0BZ, England 5.Imperial Coll London, Ctr Plast Elect, London W12 0BZ, England 6.Lanzhou Univ, Coll Chem & Chem Engn, State Key Lab Appl & Organ Chem, Lanzhou 730000, Peoples R China |
| 推荐引用方式 GB/T 7714 | Liang, Xianfeng,Chen, Yanlin,Jiao, Xuechen,et al. Vinylene Flanked Naphtho[1,2-c:5,6-c ']bis[1,2,5]thiadiazole Polymer for Low-Crystallinity Ambipolar Transistors[J]. MACROMOLECULES,2022,55(1):331-337. |
| APA | Liang, Xianfeng.,Chen, Yanlin.,Jiao, Xuechen.,Heeney, Martin.,McNeill, Christopher R..,...&Tan, Luxi.(2022).Vinylene Flanked Naphtho[1,2-c:5,6-c ']bis[1,2,5]thiadiazole Polymer for Low-Crystallinity Ambipolar Transistors.MACROMOLECULES,55(1),331-337. |
| MLA | Liang, Xianfeng,et al."Vinylene Flanked Naphtho[1,2-c:5,6-c ']bis[1,2,5]thiadiazole Polymer for Low-Crystallinity Ambipolar Transistors".MACROMOLECULES 55.1(2022):331-337. |
入库方式： OAI收割
来源：重庆绿色智能技术研究院
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