One step methane production based on catalytic pressurized calcium looping gasification with in-situ CO2 capture and self-sustained heat supply
文献类型：期刊论文
| 作者 | Zhou, Xing6,7; Yang, Xin5; Zheng, Jie4; Li, Junguo3; Li, Haibin1 ; Fang, Yitian2,6; Yu, Zhongliang4,6
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| 刊名 | JOURNAL OF THE ENERGY INSTITUTE
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| 出版日期 | 2021-12-01 |
| 卷号 | 99页码:256-265 |
| 关键词 | Calcium looping Steam hydrogasification Methane production Autothermal gasification |
| ISSN号 | 1743-9671 |
| DOI | 10.1016/j.joei.2021.10.002 |
| 通讯作者 | Yu, Zhongliang(yzh2401@126.com) |
| 英文摘要 | Catalytic steam hydrogasification of coal is a direct method for methane production. Calcium looping concept is usually used in coal gasification process for in-situ carbon dioxide removal and heat supply. In this paper, a new process combining catalytic steam hydrogasification and calcium looping was proposed and investigated using a self designed instantaneously feeding reactor under high-temperature and pressurized conditions. The effects of operation conditions (including hydrogen concentration with a range of 0-50 vol%, gasification pressure with a range of 0.1-3.5 MPa, gasification temperature with a range of 700-800 degrees C, and gasification-calcination cycle number up to six) on the performance of the new process have been studied. The results show that: (i) increasing H-2 concentration is beneficial to methane products; (ii) high temperature and low pressure are not conducive to methane production and carbon dioxide capture as well as the self-sustained heat supply in gasifier; (iii) the methane content and carbon conversion can be maintained at 30-40 vol% and 75-80% for the durability tests. According to the performance of gas products, 750 degrees C 3.5 MPa and Ca/C = 0.5 are suggested for the new process. In addition, the gasification reactivity can be affected by the Ca-K-Char interaction as indicated by the XRD, FTIR and SEM-EDX analysis. |
| WOS关键词 | QUALITY SYNGAS PRODUCTION ; COAL-GASIFICATION ; CHAR GASIFICATION ; GAS-PRODUCTION ; FLUIDIZED-BED ; PYROLYSIS ; HYDROGASIFICATION ; SORBENTS ; BIOMASS ; TAR |
| WOS研究方向 | Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:000712078700001 |
| 出版者 | ELSEVIER SCI LTD |
| 源URL | [http://ir.giec.ac.cn/handle/344007/35180]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Yu, Zhongliang |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 2.Chinese Acad Sci, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China 3.Southern Univ Sci & Technol, Acad Adv Interdisciplinary Studies, Dept Chem, Shenzhen 518055, Peoples R China 4.Shangrao Normal Univ, Sch Chem & Environm Sci, Shangrao 334001, Peoples R China 5.Univ Oxford, Dept Engn Sci, Oxford OX2 0ES, England 6.Chinese Acad Sci, Inst Coal Chem, State Key Lab Coal Convers, Taiyuan 030001, Peoples R China 7.Hebei Normal Univ, Coll Engn, Shijiazhuang 050024, Hebei, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhou, Xing,Yang, Xin,Zheng, Jie,et al. One step methane production based on catalytic pressurized calcium looping gasification with in-situ CO2 capture and self-sustained heat supply[J]. JOURNAL OF THE ENERGY INSTITUTE,2021,99:256-265. |
| APA | Zhou, Xing.,Yang, Xin.,Zheng, Jie.,Li, Junguo.,Li, Haibin.,...&Yu, Zhongliang.(2021).One step methane production based on catalytic pressurized calcium looping gasification with in-situ CO2 capture and self-sustained heat supply.JOURNAL OF THE ENERGY INSTITUTE,99,256-265. |
| MLA | Zhou, Xing,et al."One step methane production based on catalytic pressurized calcium looping gasification with in-situ CO2 capture and self-sustained heat supply".JOURNAL OF THE ENERGY INSTITUTE 99(2021):256-265. |
入库方式： OAI收割
来源：广州能源研究所
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