Influence of Direct Current-Voltage Accompanied by Charge Flow on CO2 Hydrate Formation
文献类型：期刊论文
| 作者 | Zhao, Qi1,2,3,4; Xia, Zhi-Ming1,2,3; Xu, Chun-Gang1,2,3; Chen, Zhao-Yang1,2,3; Li, Xiao-Sen1,2,3,4
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| 刊名 | FRONTIERS IN ENERGY RESEARCH
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| 出版日期 | 2021-11-15 |
| 卷号 | 9页码:11 |
| 关键词 | carbon dioxide gas hydrate direct current-voltage charge flow kinetics |
| ISSN号 | 2296-598X |
| DOI | 10.3389/fenrg.2021.770599 |
| 通讯作者 | Xia, Zhi-Ming(xiazm@ms.giec.ac.cn) ; Li, Xiao-Sen(lixs@ms.giec.ac.cn) |
| 英文摘要 | The capture and storage of carbon dioxide (CO2) are urgent and crucial to achieve the goal of carbon neutrality. Hydrate-based CO2 capture technology is one of the promising technologies for capturing and storing CO2. This work studied the nucleation and growth of CO2 hydrate provoked by direct current-voltage accompanied by charge flow with the agitation of 450 rpm at an initial pressure of 3.5 MPa and a temperature of 274.15 K. The results show that the physical bubble behavior and electrochemistry mechanisms could influence CO2 hydrate formation process in the application of voltage. The induction time and semi-completion time of CO2 hydrate formation were decreased by 51% and 27.8% in the presence of 15 V, respectively. However, more product of electrolysis, Joule heat and ions, could inhibit the CO2 hydrate formation process in the application of a high voltage (60 V). In addition, a high voltage (60 V) could change the morphology characteristics of CO2 hydrate from gel-like to whisker-like. This study provides valuable information on the formation of CO2 hydrate under the action of charge flow. |
| WOS关键词 | ELECTRIC-FIELD ; WATER ; CAPTURE ; KINETICS ; METHANE ; NUCLEATION ; ELECTRONUCLEATION |
| 资助项目 | Key Program of National Natural Science Foundation of China[51736009] ; National Natural Science Foundation of China[51879254] ; Fundamental Research and Applied Fundamental Research Major Project of Guangdong Province[2019B030302004] ; Fundamental Research and Applied Fundamental Research Major Project of Guangdong Province[2020B0301030003] ; Guangdong Special Support Program-Local innovation and entrepreneurship team project[2019BT02L278] ; Special Project for Marine Economy Development of Guangdong Province[GDME-2018D002] ; Special Project for Marine Economy Development of Guangdong Province[GDME-2020D044] ; National Natural Science Foundation of Guangdong[2019A1515011730] |
| WOS研究方向 | Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:000726071500001 |
| 出版者 | FRONTIERS MEDIA SA |
| 资助机构 | Key Program of National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research and Applied Fundamental Research Major Project of Guangdong Province ; Guangdong Special Support Program-Local innovation and entrepreneurship team project ; Special Project for Marine Economy Development of Guangdong Province ; National Natural Science Foundation of Guangdong |
| 源URL | [http://ir.giec.ac.cn/handle/344007/35376]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Xia, Zhi-Ming; Li, Xiao-Sen |
| 作者单位 | 1.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou, Peoples R China 2.Chinese Acad Sci, Key Lab Gas Hydrate, Guangzhou Inst Energy Convers, Guangzhou, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou, Peoples R China 4.Univ Sci & Technol China, Sch Engn Sci, Dept Thermal Sci & Energy Engn, Hefei, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Qi,Xia, Zhi-Ming,Xu, Chun-Gang,et al. Influence of Direct Current-Voltage Accompanied by Charge Flow on CO2 Hydrate Formation[J]. FRONTIERS IN ENERGY RESEARCH,2021,9:11. |
| APA | Zhao, Qi,Xia, Zhi-Ming,Xu, Chun-Gang,Chen, Zhao-Yang,&Li, Xiao-Sen.(2021).Influence of Direct Current-Voltage Accompanied by Charge Flow on CO2 Hydrate Formation.FRONTIERS IN ENERGY RESEARCH,9,11. |
| MLA | Zhao, Qi,et al."Influence of Direct Current-Voltage Accompanied by Charge Flow on CO2 Hydrate Formation".FRONTIERS IN ENERGY RESEARCH 9(2021):11. |
入库方式： OAI收割
来源：广州能源研究所
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