Graphene-assisted construction of electrocatalysts for carbon dioxide reduction
文献类型：期刊论文
| 作者 | Hu, Huawen6; Ou, Jian Zhen5,6; Xu, Xuejun6; Lin, Yinlei6; Zhang, Yuyuan6; Zhao, Hong6; Chen, Dongchu6; He, Minghui4; Huang, Yugang2,3; Deng, Lifang1 |
| 刊名 | CHEMICAL ENGINEERING JOURNAL
 |
| 出版日期 | 2021-12-01 |
| 卷号 | 425页码:26 |
| 关键词 | Graphene Electrocatalysts CO2 reduction Metal-based Non-metal Active sites |
| ISSN号 | 1385-8947 |
| DOI | 10.1016/j.cej.2021.130587 |
| 通讯作者 | Ou, Jian Zhen(Jianzhen.ou@rmit.edu.au) |
| 英文摘要 | The electrochemical conversion of the greenhouse gas, carbon dioxide (CO2), to energy fuels and value-added chemicals presents one of the most valuable approaches to harvest pollutants and produce renewable energy. However, the stable molecular structure of CO2 and the sluggish reaction kinetics make CO2 reduction reaction (CO2RR) formidably challenging to achieve reaction rate and selectivity practical in industry. Graphene and its derivatives have been considered a group of intriguing materials to develop advanced CO2RR electrocatalysts due to their large specific surface area, remarkable electron transfer ability, superior stability, and easy tunability of the structure and surface properties. Herein, we comprehensively discuss the state-of-the-art electrocatalysts constructed with graphene and derivatives for active and selective CO2RR within the recent five years, mainly including the electrocatalysts with both metal-based (e.g., noble, non-noble, or combined thereof) and non-metal (e.g., doped, modified, defected, or composited) catalytic sites. To present the versatile, high-performance metal-based CO2RR electrocatalysts constructed with graphene, we further subdivide them according to the sizes, oxidation states, metal species synergies, dimensionalities, and versatility. Finally, we provide the challenges and perspectives in this emerging area of utilising CO2 to produce various carbon-based fuels and chemicals via graphene chemistry. |
| WOS关键词 | NITROGEN-DOPED GRAPHENE ; EFFICIENT ELECTROCHEMICAL REDUCTION ; CO2 ELECTROREDUCTION PERFORMANCE ; METAL-FREE ELECTROCATALYST ; SINGLE-ATOM CATALYSTS ; OXYGEN REDUCTION ; SELECTIVE ELECTROREDUCTION ; FORMIC-ACID ; OXIDE ; NANOPARTICLES |
| 资助项目 | Key-Area Special Project of Guangdong Provincial Education Department[2020ZDZX2066] ; Key Project of Guangdong Basic and Applied Basic Research Foundation[2020B1515120081] ; National Natural Science Foundation of China[51906045] ; National Natural Science Foundation of China[51803028] ; Key-Area Research and Development Program Project of Guangdong Province[2020B0909040002] ; National Natural Science Foundation of Guangdong Province[2019A1515010928] |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000707126000064 |
| 出版者 | ELSEVIER SCIENCE SA |
| 资助机构 | Key-Area Special Project of Guangdong Provincial Education Department ; Key Project of Guangdong Basic and Applied Basic Research Foundation ; National Natural Science Foundation of China ; Key-Area Research and Development Program Project of Guangdong Province ; National Natural Science Foundation of Guangdong Province |
| 源URL | [http://ir.giec.ac.cn/handle/344007/35385]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Ou, Jian Zhen |
| 作者单位 | 1.Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China 2.Guangzhou Med Univ, Sch Pharmaceut Sci, Guangzhou 511436, Guangdong, Peoples R China 3.Guangzhou Med Univ, Key Lab Mol Target & Clin Pharmacol, Guangzhou 511436, Guangdong, Peoples R China 4.South China Univ Technol, Sch Light Ind & Engn, State Key Lab Pulp & Paper Engn, Guangzhou 510640, Guangdong, Peoples R China 5.RMIT Univ, Sch Engn, Melbourne, Vic 3000, Australia 6.Foshan Univ, Sch Mat Sci & Hydrogen Energy, Foshan 528000, Guangdong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Hu, Huawen,Ou, Jian Zhen,Xu, Xuejun,et al. Graphene-assisted construction of electrocatalysts for carbon dioxide reduction[J]. CHEMICAL ENGINEERING JOURNAL,2021,425:26. |
| APA | Hu, Huawen.,Ou, Jian Zhen.,Xu, Xuejun.,Lin, Yinlei.,Zhang, Yuyuan.,...&Deng, Lifang.(2021).Graphene-assisted construction of electrocatalysts for carbon dioxide reduction.CHEMICAL ENGINEERING JOURNAL,425,26. |
| MLA | Hu, Huawen,et al."Graphene-assisted construction of electrocatalysts for carbon dioxide reduction".CHEMICAL ENGINEERING JOURNAL 425(2021):26. |
入库方式： OAI收割
来源：广州能源研究所
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