Interfacial Reaction Between Nickel-Based Superalloy K417G and Oxide Refractories
文献类型：期刊论文
| 作者 | Song Qingzhong2,3; Qian Kun1,3; Shu Lei1,3; Chen Bo1,3; Ma Yingche1,3; Liu Kui1,3 |
| 刊名 | ACTA METALLURGICA SINICA
 |
| 出版日期 | 2022-07-11 |
| 卷号 | 58期号:7页码:868-882 |
| ISSN号 | 0412-1961 |
| 关键词 | interfacial reaction K417G refractory Al2O3 CaO MgO ZrO2 Y2O3 |
| DOI | 10.11900/0412.1961.2021.00048 |
| 通讯作者 | Chen Bo(bchen@imr.ac.cn) |
| 英文摘要 | High-performance nickel-based superalloys are highly desired in the aerospace industry. A drawback of vacuum induction melting for processing nickel-based superalloys is that oxide refractories contaminate the molten alloy through crucible-melt interaction. Therefore, crucibles used for producing nickel-based superalloys should be carefully selected to avoid melt contamination. In this study, the interfacial reaction between a molten nickel-based superalloy (K417G) and various oxide refractories, including Al2O3, CaO, MgO, ZrO2 + 12%Y2O3 (mass fraction) (Y-PSZ), ZrO2 + 20%CaO (CSZ), and Y2O3, formed by cold isostatic pressing was investigated at 1600 degrees C by XRD, SEM, and EDS. The effects of the oxide crucibles on the impurity contents of K417G were also evaluated. The results show that physical erosion is the primary mechanism of the interaction between Al2O3 crucibles and alloy melt. The readily detached Al2O3 particles formed inclusions in the alloy. The Ca3Al2O5 liquid phase generated at the melt-crucible interface promoted wettability between the alloy and CaO crucible, resulting in a high adhesion at the interface. The reaction of the MgO crucible with Al in the alloy resulted in the formation of MgAl2O4 at the melt-crucible interface, which subsequently entered the alloy to form inclusions. Al2O3 was generated at the Y-PSZ-crucible-alloy interface. However, there was no corrosion of Al2O3 in the Y-PSZ crucible, indicating the crucible exhibits excellent corrosion resistance to Al2O3 slags. The interaction between the CSZ crucible and alloy melt generated a CaAl2O4 liquid phase, making the crucible unstable to dissolve into the alloy. An Al2Y4O9 reaction layer is mainly formed at the Y2O3-crucible-alloy interface. The dissolution of Y2O3 into the alloy melt was high compared to that of other oxide refractories. The melt-crucible interaction also significantly affected the oxygen content of K417G. The oxygen concentration of the alloy fused by CaO, Y2O3, and Y-PSZ crucibles did not increase, whereas that of the alloy melted in CSZ, MgO, and Al2O3 crucibles increased from 0.0007% to 0.0011%, 0.0034%, and 0.0135%, respectively. |
| WOS研究方向 | Metallurgy & Metallurgical Engineering |
| 语种 | 英语 |
| 出版者 | SCIENCE PRESS |
| WOS记录号 | WOS:000816121700003 |
| 源URL | [http://ir.imr.ac.cn/handle/321006/174771]  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Chen Bo |
| 作者单位 | 1.Chinese Acad Sci, Shi Changxu Innovat Ctr Adv Mat, Inst Met Res, Shenyang 110016, Peoples R China 2.Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Shenyang 110016, Peoples R China |
| 推荐引用方式 GB/T 7714 | Song Qingzhong,Qian Kun,Shu Lei,et al. Interfacial Reaction Between Nickel-Based Superalloy K417G and Oxide Refractories[J]. ACTA METALLURGICA SINICA,2022,58(7):868-882. |
| APA | Song Qingzhong,Qian Kun,Shu Lei,Chen Bo,Ma Yingche,&Liu Kui.(2022).Interfacial Reaction Between Nickel-Based Superalloy K417G and Oxide Refractories.ACTA METALLURGICA SINICA,58(7),868-882. |
| MLA | Song Qingzhong,et al."Interfacial Reaction Between Nickel-Based Superalloy K417G and Oxide Refractories".ACTA METALLURGICA SINICA 58.7(2022):868-882. |
入库方式： OAI收割
来源：金属研究所
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