Synthesis, Characterization, and Dye Removal of ZnCl2-Modified Biochar Derived from Pulp and Paper Sludge
文献类型：期刊论文
| 作者 | Zhao, Fengxiao3,4,5,6; Shan, Rui4,5,6; Li, Wenjian2; Zhang, Yuyuan1; Yuan, Haoran4,5,6 ; Chen, Yong4,5,6
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| 刊名 | ACS OMEGA
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| 出版日期 | 2021-12-10 |
| 页码 | 12 |
| ISSN号 | 2470-1343 |
| DOI | 10.1021/acsomega.1c05142 |
| 通讯作者 | Yuan, Haoran(yuanhr@ms.giec.ac.cn) |
| 英文摘要 | In this study, pulp sludge-derived biochar synthesized through modification with ZnCl2 under multistep pyrolysis conditions was investigated for the effective removal of methylene blue (MB) from aqueous solution. Results showed that when the Zn2PT350-700 dosage was 10 mg, the largest adsorption amount of MB was 590.20 mg/g within 24 h under pH = 8. Kinetics and thermodynamics revealed that the adsorption process of MB can be described by the Freundlich isotherm model and the pseudo-second-order kinetic model, which means that multilayer sorption occurred on the heterogeneous surface of Zn2PT350-700. The analysis of the adsorption mechanism showed that electrostatic attraction between the deprotonated functional groups and MB+, cation exchange, and pi-electron interaction played a major role in MB adsorption, followed by physical adsorption. After six cycles of desorption-adsorption, Zn2PT350-700 still maintained good adsorption performance. All results demonstrated that Zn2PT350700 could perform as promising adsorbents for efficient MB removal from wastewater. Using biochar from paper and pulp sludge for wastewater remediation is an ingenious method, which can reduce the environmental and health risks related to industrial waste disposal, while providing remediation of water contaminated with industrial dye effluents. |
| WOS关键词 | ACTIVATED CARBONS ; MILL SLUDGE ; ADSORPTION ; PYROLYSIS ; ADSORBENT ; WATER ; TEMPERATURE ; PERFORMANCE ; KINETICS ; ACID |
| 资助项目 | State's Key Project of Research and Development Plan, China[2020YFC1908900] ; National Natural Science Funds of China[51776211] ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou)[GML2019ZD0101] ; Science and Technology Program of Guangdong Province, China[2021A1515012263] ; Science and Technology Program of Guangdong Province, China[2019B110210003] ; Science and Technology Program of Guangzhou, China[202002030365] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000731116200001 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | State's Key Project of Research and Development Plan, China ; National Natural Science Funds of China ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou) ; Science and Technology Program of Guangdong Province, China ; Science and Technology Program of Guangzhou, China |
| 源URL | [http://ir.giec.ac.cn/handle/344007/35470]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Yuan, Haoran |
| 作者单位 | 1.Coll Mat Sci & Energy Engn, Foshan 528000, Peoples R China 2.Zhejiang Golden Pot Boiler Ltd, Jinhua 321015, Zhejiang, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 4.CAS Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 5.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China 6.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Fengxiao,Shan, Rui,Li, Wenjian,et al. Synthesis, Characterization, and Dye Removal of ZnCl2-Modified Biochar Derived from Pulp and Paper Sludge[J]. ACS OMEGA,2021:12. |
| APA | Zhao, Fengxiao,Shan, Rui,Li, Wenjian,Zhang, Yuyuan,Yuan, Haoran,&Chen, Yong.(2021).Synthesis, Characterization, and Dye Removal of ZnCl2-Modified Biochar Derived from Pulp and Paper Sludge.ACS OMEGA,12. |
| MLA | Zhao, Fengxiao,et al."Synthesis, Characterization, and Dye Removal of ZnCl2-Modified Biochar Derived from Pulp and Paper Sludge".ACS OMEGA (2021):12. |
入库方式： OAI收割
来源：广州能源研究所
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