New mechanistic insight into rapid adsorption of pharmaceuticals from water utilizing activated biochar
文献类型：期刊论文
| 作者 | Maged, Ali2,3; Dissanayake, Pavani Dulanja4,5,6; Yang, Xiao7; Pathirannahalage, Charitha2; Bhatnagar, Amit1,2; Ok, Yong Sik4,5 |
| 刊名 | ENVIRONMENTAL RESEARCH
 |
| 出版日期 | 2021-11-01 |
| 卷号 | 202页码:15 |
| 关键词 | Diclofenac Levofloxacin Biochar Adsorption Water treatment Waste valorization |
| ISSN号 | 0013-9351 |
| DOI | 10.1016/j.envres.2021.111693 |
| 通讯作者 | Maged, Ali(Ali.Maged@suezuni.edu.eg) ; Bhatnagar, Amit(amit.bhatnagar@lut.fi) ; Ok, Yong Sik(yongsikok@korea.ac.kr) |
| 英文摘要 | The presence of emerging pollutants especially hazardous chemicals and pharmaceuticals in aquatic environments is a matter of grave concern to human health and the environment. In this study, coffee bean waste (CBW) was utilized to synthesize pristine (CBW550) and activated (CBWHPO550 ) biochars for the elimination of diclofenac (DF) and levofloxacin (LEV) from water. A facile two-step approach was used to synthesize CBWHPO 550 using chemical pretreatment and pyrolysis under N2 purging. BET results of CBWHPO 550 revealed that chemical pretreatment increased surface area by approximately 160 times compared to CBW550. The calculated ID/IG ratio from Raman spectra confirmed that CBWHPO550 had a high functionalized surface. Different operational parameters such as contact time, pH, adsorbent dose, ionic strength, and adsorbate concentration were studied and optimized. Maximum Langmuir adsorption capacity of CBWHPO 550 was found to be 61.17 and 110.70 mg/g for DF and LVX, respectively. Experimental results demonstrated that presence of NaCl in solution enhanced DF removal efficiency due to the salting-out effect. Electrostatic attraction, pi - pi bonding, and hydrophobic interaction were prominently responsible mechanisms for the adsorption of DF and LVX. Furthermore, continuous-flow mode studies confirmed that CBWHPO |
| WOS关键词 | FIXED-BED COLUMN ; SPENT COFFEE GROUNDS ; AQUEOUS-SOLUTION ; DICLOFENAC SODIUM ; TREATMENT PLANTS ; ORGANIC CONTAMINANTS ; GRAPHENE OXIDE ; REMOVAL ; CARBON ; LEVOFLOXACIN |
| 资助项目 | Cooperative Research Program for Agriculture Science and Technology Development (Effects of plastic mulch wastes on crop productivity and agroenvironment), Rural Development Administration, Republic of Korea[PJ01475801] ; National Research Foundation of Korea (NRF) - Korea government (MSIT)[2021R1A2C2011734] |
| WOS研究方向 | Environmental Sciences & Ecology ; Public, Environmental & Occupational Health |
| 语种 | 英语 |
| WOS记录号 | WOS:000704657900003 |
| 出版者 | ACADEMIC PRESS INC ELSEVIER SCIENCE |
| 资助机构 | Cooperative Research Program for Agriculture Science and Technology Development (Effects of plastic mulch wastes on crop productivity and agroenvironment), Rural Development Administration, Republic of Korea ; National Research Foundation of Korea (NRF) - Korea government (MSIT) |
| 源URL | [http://ir.igsnrr.ac.cn/handle/311030/166896]  |
| 专题 | 中国科学院地理科学与资源研究所 |
| 通讯作者 | Maged, Ali; Bhatnagar, Amit; Ok, Yong Sik |
| 作者单位 | 1.LUT Univ, LUT Sch Engn Sci, Dept Separat Sci, Sammonkatu 12, FI-50130 Mikkeli, Finland 2.Univ Eastern Finland, Dept Environm & Biol Sci, POB 1627, FI-70211 Kuopio, Finland 3.Suez Univ, Fac Sci, Geol Dept, POB 43518, El Salam City, Suez Governorat, Egypt 4.Korea Univ, Korea Biochar Res Ctr, APRU Sustainable Waste Management Program, Seoul 02841, South Korea 5.Korea Univ, Div Environm Sci & Ecol Engn, Seoul 02841, South Korea 6.Coconut Res Inst, Soils & Plant Nutr Div, Lunuwila 61150, Sri Lanka 7.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Key Lab Land Surface Pattern & Simulat, Beijing 100101, Peoples R China |
| 推荐引用方式 GB/T 7714 | Maged, Ali,Dissanayake, Pavani Dulanja,Yang, Xiao,et al. New mechanistic insight into rapid adsorption of pharmaceuticals from water utilizing activated biochar[J]. ENVIRONMENTAL RESEARCH,2021,202:15. |
| APA | Maged, Ali,Dissanayake, Pavani Dulanja,Yang, Xiao,Pathirannahalage, Charitha,Bhatnagar, Amit,&Ok, Yong Sik.(2021).New mechanistic insight into rapid adsorption of pharmaceuticals from water utilizing activated biochar.ENVIRONMENTAL RESEARCH,202,15. |
| MLA | Maged, Ali,et al."New mechanistic insight into rapid adsorption of pharmaceuticals from water utilizing activated biochar".ENVIRONMENTAL RESEARCH 202(2021):15. |
入库方式： OAI收割
来源：地理科学与资源研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。