Composition and sources of particulate matter in the Beijing-Tianjin-Hebei region and its surrounding areas during the heating season
文献类型:期刊论文
作者 | Dao, Xu1; Di, Shiying1; Zhang, Xian1; Gao, Panjun2; Wang, Li3; Yan, Luyu1; Tang, Guigang1; He, Lihuan1; Krafft, Thomas2; Zhang, Fengying1,2 |
刊名 | CHEMOSPHERE |
出版日期 | 2022-03-01 |
卷号 | 291页码:10 |
ISSN号 | 0045-6535 |
关键词 | Heating season Particulate matter PM components Source analysis |
DOI | 10.1016/j.chemosphere.2021.132779 |
通讯作者 | Zhang, Fengying(zhangfy@cnemc.cn) |
英文摘要 | This paper aimed to analyze the composition and pollution sources of particulate matter (PM) in the BeijingTianjin-Hebei region and its surrounding areas (henceforth the BTH region) during the heating season to support the mitigation and control of regional air pollution. Manual monitoring data from the China National Environmental Monitoring Network for Atmospheric PM in the BTH region were collected and analyzed during the 2016 and 2018 heating seasons. The positive definite matrix factor analysis (PMF) model was used to analyze the PM sources in BTH cities during the heating season. The main PM components were organic matter (OM), nitrate (NO3-), sulfate (SO42-) and ammonium salt (NH4+). Direct emission sources have decreased since 2016, indicating the effectiveness of governmental controls on these sources; however, secondary pollution showed an increasing trend, suggesting control measures should be strengthened. Daily regional average concentrations of OM, SO42-, NH4+, elemental carbon (EC), chloride (Cl-) and trace elements all showed similar trends. When air quality worsened, the concentrations of the main PM components increased, but trends of change varied among components. In 2018, concentrations of OM and chloride were highest in the Taihang Mountains, and NO3 concentrations were highest in Anyang, Hebi, Jiaozuo and Xinxiang. The SO42- concentration was highest in the southern section of the Taihang Mountains. The NH4+ and EC concentrations were generally highest in the central and southern regions. The concentration of crustal substances was highest in some cities in the north and central parts of the BTH region. In the 2018 heating season, the pollution level of five transmission channels showed an increasing trend in the Northwest, Southeast, Yanshan, South and Taihang Mountain channels. These findings provide a scientific basis for the continued management of atmospheric PM pollution. |
WOS关键词 | POSITIVE MATRIX FACTORIZATION ; CHEMICAL-COMPOSITION ; AMBIENT PM2.5 ; SOURCE APPORTIONMENT ; HEALTH IMPACT ; MORTALITY ; BURDEN ; VARIABILITY ; CHINA |
资助项目 | Strategic Priority Research Program of Chinese Academy of Sciences[XDA23100400] ; National Natural Science Foundation of China[41401101] ; Shanghai Key Lab for Urban Ecological Processes and Eco-Restoration[SHUES 2019A10] |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
WOS记录号 | WOS:000757882300006 |
资助机构 | Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; Shanghai Key Lab for Urban Ecological Processes and Eco-Restoration |
源URL | [http://ir.igsnrr.ac.cn/handle/311030/170822] |
专题 | 中国科学院地理科学与资源研究所 |
通讯作者 | Zhang, Fengying |
作者单位 | 1.China Natl Environm Monitoring Ctr, Beijing 100012, Peoples R China 2.Maastricht Univ, Fac Hlth Med & Life Sci, CAPHRI Care & Publ Hlth Res Inst, Dept Hlth Eth & Soc, Maastricht, Netherlands 3.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China |
推荐引用方式 GB/T 7714 | Dao, Xu,Di, Shiying,Zhang, Xian,et al. Composition and sources of particulate matter in the Beijing-Tianjin-Hebei region and its surrounding areas during the heating season[J]. CHEMOSPHERE,2022,291:10. |
APA | Dao, Xu.,Di, Shiying.,Zhang, Xian.,Gao, Panjun.,Wang, Li.,...&Zhang, Fengying.(2022).Composition and sources of particulate matter in the Beijing-Tianjin-Hebei region and its surrounding areas during the heating season.CHEMOSPHERE,291,10. |
MLA | Dao, Xu,et al."Composition and sources of particulate matter in the Beijing-Tianjin-Hebei region and its surrounding areas during the heating season".CHEMOSPHERE 291(2022):10. |
入库方式: OAI收割
来源:地理科学与资源研究所
浏览0
下载0
收藏0
其他版本
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。