Organosilicon-Based Functional Electrolytes for High-Performance Lithium Batteries
文献类型：期刊论文
| 作者 | Wang, Hualan; Chen, Shuangxi; Li, Yan; Liu, Yongfeng; Jing, Qiuju; Liu, Xue; Liu, Zhaoping; Zhang, Xiaogang |
| 刊名 | ADVANCED ENERGY MATERIALS
 |
| 出版日期 | 2021 |
| 卷号 | 11期号:28 |
| 关键词 | SOLID POLYMER ELECTROLYTES POLYHEDRAL OLIGOMERIC SILSESQUIOXANE PASSIVE FILM FORMATION LI-S BATTERIES POLYSILOXANE-BASED ELECTROLYTE IONIC LIQUIDS DI-UREASILS TRIS(TRIMETHYLSILYL) PHOSPHITE ELECTROCHEMICAL PROPERTIES COMPOSITE ELECTROLYTES |
| 英文摘要 | The electrolyte has been considered as a key factor toward higher energy density for Li-ion and Li-metal batteries. However, conventional electrolytes suffer from uncontrolled interfacial reactions and irreversible decomposition causing performance deterioration and potential safety hazard. Organosilicon compounds have attracted great interest as promising electrolyte components due to facile chemical modifications, low glass transition temperatures (T-g), superior chemical, and thermal stabilities. Considerable investigation efforts have been devoted to developing better overall performance of organosilicon-based electrolytes in the past few years. Herein, the recent research progress of organosilicon-based functional electrolytes for the development of liquid, gel, and solid state electrolytes in Li-ion and Li-metal batteries is summarized. Attention is devoted to various types of organosilicon such as silane, siloxane, polysiloxane, and polyhedral oligomeric silsesquioxanes in terms of molecular design, ionic conductivity, functions shown in batteries, thermal, chemical, electrochemical stability, safety, etc. The feasible strategies are also discussed that may promote the comprehensive electrochemical performances of organosilicon-based electrolytes in different types of electrolytes and batteries. Finally, the challenges facing organosilicon-based electrolytes and proposed their possible solutions are presented alongside promising development directions. |
| 源URL | [http://ir.nimte.ac.cn/handle/174433/21840]  |
| 专题 | 中国科学院宁波材料技术与工程研究所 2021专题_期刊论文 |
| 作者单位 | 1.Zhang, XG (corresponding author), Nanjing Univ Aeronaut & Astronaut, Jiangsu Key Lab Electrochem Energy Storage Techno, Coll Mat Sci & Technol, Nanjing 210016, Peoples R China. 2.Li, Y (corresponding author), Hangzhou Normal Univ, Minist Educ, Key Lab Organosilicon Chem & Mat Technol, Hangzhou 311121, Peoples R China. 3.Liu, YF (corresponding author), Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China. 4.Liu, YF (corresponding author), Zhejiang Univ, Sch Mat Sci & Engn, Hangzhou 310027, Peoples R China. 5.Liu, ZP (corresponding author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Adv Li Ion Battery Engn Lab Zhejiang Prov, CAS Engn Lab Graphene,Key Lab Graphene Technol &, Ningbo 315201, Peoples R China. |
| 推荐引用方式 GB/T 7714 | Wang, Hualan,Chen, Shuangxi,Li, Yan,et al. Organosilicon-Based Functional Electrolytes for High-Performance Lithium Batteries[J]. ADVANCED ENERGY MATERIALS,2021,11(28). |
| APA | Wang, Hualan.,Chen, Shuangxi.,Li, Yan.,Liu, Yongfeng.,Jing, Qiuju.,...&Zhang, Xiaogang.(2021).Organosilicon-Based Functional Electrolytes for High-Performance Lithium Batteries.ADVANCED ENERGY MATERIALS,11(28). |
| MLA | Wang, Hualan,et al."Organosilicon-Based Functional Electrolytes for High-Performance Lithium Batteries".ADVANCED ENERGY MATERIALS 11.28(2021). |
入库方式： OAI收割
来源：宁波材料技术与工程研究所
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