Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting
文献类型：期刊论文
| 作者 | Yuan, Cheng-Zong; Hui, Kwan San; Yin, Hong; Zhu, Siqi; Zhang, Jintao; Wu, Xi-Lin; Hong, Xiaoting; Zhou, Wei; Fan, Xi; Bin, Feng |
| 刊名 | ACS MATERIALS LETTERS
 |
| 出版日期 | 2021 |
| 卷号 | 3期号:6页码:752-780 |
| 关键词 | HYDROGEN EVOLUTION REACTION NITROGEN-DOPED CARBON EFFICIENT BIFUNCTIONAL ELECTROCATALYST LAYERED DOUBLE HYDROXIDE SINGLE-ATOM CATALYSTS HIGH-SURFACE-AREA IN-SITU FORMATION OXYGEN EVOLUTION COBALT OXIDE ACTIVE-SITES |
| 英文摘要 | Efficient and low-cost transition-metal (TM)-based electrocatalysts have been of great importance for producing hydrogen (H-2) and oxygen (O-2) via electrocatalytic water (H2O) splitting to ameliorate global energy and environmental problems. However, TM-based materials generally suffer from unsatisfactory electrocatalytic activity because of their relatively low conductivity and unregulated electronic structure. Therefore, the electronic structure engineering of electrocatalysts is an efficient strategic approach to enhance catalytic performances and stabilities. In this review, recent experimental and theoretical advances in the intrinsic electronic structure regulation of TM-based nanomaterials are summarized in terms of preparation methods and underlying natures to boost hydrogen evolution reaction and oxygen evolution reaction. A systematic discussion is conducted on engineering strategies for TM-based nanomaterials to regulate their electronic structures, optimize their adsorption ability of reaction intermediates, and reduce reaction barrier. The existing challenges and perspectives of TM-based electrocatalysts are highlighted to provide new insights into technological advancement for hydrogen production. |
| 源URL | [http://ir.nimte.ac.cn/handle/174433/21842]  |
| 专题 | 中国科学院宁波材料技术与工程研究所 2021专题_期刊论文 |
| 作者单位 | 1.Hui, KS (corresponding author), Univ East Anglia, Fac Sci, Sch Engn, Norwich NR4 7TJ, Norfolk, England. 2.Chen, FM (corresponding author), South China Normal Univ, Sch Phys & Telecommun Engn, State Key Lab Opt Informat Phys & Technol, Guangzhou 510006, Peoples R China. 3.Hui, KN (corresponding author), Univ Macau, Inst Appl Phys & Mat Engn, Minist Educ, Joint Key Lab, Taipa 999078, Macau Sar, Peoples R China. |
| 推荐引用方式 GB/T 7714 | Yuan, Cheng-Zong,Hui, Kwan San,Yin, Hong,et al. Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting[J]. ACS MATERIALS LETTERS,2021,3(6):752-780. |
| APA | Yuan, Cheng-Zong.,Hui, Kwan San.,Yin, Hong.,Zhu, Siqi.,Zhang, Jintao.,...&Hui, Kwun Nam.(2021).Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting.ACS MATERIALS LETTERS,3(6),752-780. |
| MLA | Yuan, Cheng-Zong,et al."Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting".ACS MATERIALS LETTERS 3.6(2021):752-780. |
入库方式： OAI收割
来源：宁波材料技术与工程研究所
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