Zr-MOFs loaded on polyurethane foam by polydopamine for enhanced dye adsorption
文献类型:期刊论文
作者 | Zhao, Jingjing; Xu, Linqiong; Su, Yaozhuo; Yu, Hongwei; Liu, Hui; Qian, Shaoping; Zheng, Wenge; Zhao, Yongqing |
刊名 | JOURNAL OF ENVIRONMENTAL SCIENCES
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出版日期 | 2021 |
卷号 | 101页码:177-188 |
关键词 | METAL-ORGANIC FRAMEWORK RARE-EARTH-ELEMENTS SIMULTANEOUS REMOVAL WASTE-WATER COMPOSITE MEMBRANES EFFICIENT REMOVAL SEPARATION UIO-66 CO2 RECOVERY |
英文摘要 | Zirconium-based metal-organic frameworks (Zr-MOFs) have attracted widespread attention due to their high specific surface area, high porosity, abundant metal active sites and excellent hydrothermal stability. However, Zr-MOFs materials are mostly powdery in nature and thus difficult to separate from aqueous media, which limits their application in wastewater treatment. In this study, PDA/Zr-MOFs/PU foam was constructed by growing Zr-MOFs nanoparticles on a dopamine-modified polyurethane foam substrate by in-situ hydrothermal synthesis as an adsorbent for removing dyes from wastewater. The results demonstrated that the polydopamine coating improves the dispersion of the Zr-MOFs nanoparticles on the substrate and enhances the interaction between the Zr-MOFs nanoparticles and the PU foam substrate. As a result, compared with Zr-MOFs/PU foam, the prepared PDA/ZrMOFs/PU foam exhibits higher adsorption capacity for crystal violet (CV) (63.38 mg/g) and rhodamine B (RB) (67.73 mg/g), with maximum adsorption efficiencies of CV and RB of 98.4% (pH=11) and 93.5% (pH=7), respectively, at a concentration of 10 mg/L. The PDA/Zr-MOFs/PU foam can simultaneously remove CV and RB from the mixed solution. Moreover, the PDA/ZrMOFs/PU foam still exhibits high stability and reusability after five cycles. (C) 2020 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V. |
源URL | [http://ir.nimte.ac.cn/handle/174433/22159] ![]() |
专题 | 中国科学院宁波材料技术与工程研究所 2021专题_期刊论文 |
作者单位 | 1.Xu, LQ (corresponding author), Ningbo Univ, Sch Mat Sci & Chem Engn, Ningbo 315211, Peoples R China. 2.Zhao, YQ (corresponding author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo Key Lab Polymer Mat, Ningbo 315201, Peoples R China. |
推荐引用方式 GB/T 7714 | Zhao, Jingjing,Xu, Linqiong,Su, Yaozhuo,et al. Zr-MOFs loaded on polyurethane foam by polydopamine for enhanced dye adsorption[J]. JOURNAL OF ENVIRONMENTAL SCIENCES,2021,101:177-188. |
APA | Zhao, Jingjing.,Xu, Linqiong.,Su, Yaozhuo.,Yu, Hongwei.,Liu, Hui.,...&Zhao, Yongqing.(2021).Zr-MOFs loaded on polyurethane foam by polydopamine for enhanced dye adsorption.JOURNAL OF ENVIRONMENTAL SCIENCES,101,177-188. |
MLA | Zhao, Jingjing,et al."Zr-MOFs loaded on polyurethane foam by polydopamine for enhanced dye adsorption".JOURNAL OF ENVIRONMENTAL SCIENCES 101(2021):177-188. |
入库方式: OAI收割
来源:宁波材料技术与工程研究所
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