Titanium Nitride-Supported Platinum with Metal-Support Interaction for Boosting Photocatalytic H-2 Evolution of Indium Sulfide
文献类型:期刊论文
作者 | Liu, Siqi; Qi, Weiliang; Adimi, Samira; Guo, Haichuan; Weng, Bo; Attfield, John Paul; Yang, Minghui |
刊名 | ACS APPLIED MATERIALS & INTERFACES
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出版日期 | 2021 |
卷号 | 13期号:6页码:7238-7247 |
英文摘要 | Metal-support interaction strongly influences the catalytic properties of metal-based catalysts. Here, titanium nitride (TiN) nanospheres are shown to be an outstanding support, for tuning the electronic property of platinum (Pt) nanoparticles and adjusting the morphology of indium sulfide (In2S3) active components, forming flower-like core-shell nanostructures (TiN-Pt@In2S3). The strong metal-support interaction between Pt and TiN through the formation of Pt-Ti bonds favors the migration of charge carriers and leads to the easy reducibility of TiN-Pt, thus improving the photocatalytic atom efficiency of Pt. The TiN-Pt@In2S3 composite shows reduction of Pt loading by 70% compared to the optimal Pt-based system. In addition, the optimal TiN-Pt@In2S3 composite exhibits a H-2 evolution rate 4 times that of a Pt reference. This increase outperforms all other supports reported thus far. |
源URL | [http://ir.nimte.ac.cn/handle/174433/22185] ![]() |
专题 | 中国科学院宁波材料技术与工程研究所 2021专题_期刊论文 |
作者单位 | 1.Yang, MH (corresponding author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Peoples R China. 2.Yang, MH (corresponding author), Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China. 3.Attfield, JP (corresponding author), Univ Edinburgh, Sch Chem, Edinburgh EH9 3JJ, Midlothian, Scotland. 4.Weng, B (corresponding author), Katholieke Univ Leuven, cMACS, Dept Microbial & Mol Syst, B-3001 Leuven, Belgium. 5.Attfield, JP (corresponding author), Univ Edinburgh, Ctr Sci Extreme Condit, Edinburgh EH9 3JJ, Midlothian, Scotland. |
推荐引用方式 GB/T 7714 | Liu, Siqi,Qi, Weiliang,Adimi, Samira,et al. Titanium Nitride-Supported Platinum with Metal-Support Interaction for Boosting Photocatalytic H-2 Evolution of Indium Sulfide[J]. ACS APPLIED MATERIALS & INTERFACES,2021,13(6):7238-7247. |
APA | Liu, Siqi.,Qi, Weiliang.,Adimi, Samira.,Guo, Haichuan.,Weng, Bo.,...&Yang, Minghui.(2021).Titanium Nitride-Supported Platinum with Metal-Support Interaction for Boosting Photocatalytic H-2 Evolution of Indium Sulfide.ACS APPLIED MATERIALS & INTERFACES,13(6),7238-7247. |
MLA | Liu, Siqi,et al."Titanium Nitride-Supported Platinum with Metal-Support Interaction for Boosting Photocatalytic H-2 Evolution of Indium Sulfide".ACS APPLIED MATERIALS & INTERFACES 13.6(2021):7238-7247. |
入库方式: OAI收割
来源:宁波材料技术与工程研究所
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