Surface Functionalized Sensors for Humidity-Independent Gas Detection
文献类型：期刊论文
| 作者 | Qu, Fengdong; Zhang, Shendan; Huang, Chaozhu; Guo, Xuyun; Zhu, Ye; Thomas, Tiju; Guo, Haichuan; Attfield, J. Paul; Yang, Minghui |
| 刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
 |
| 出版日期 | 2021 |
| 卷号 | 60期号:12页码:6561-6566 |
| 关键词 | METAL-ORGANIC FRAMEWORKS SENSING PROPERTIES PERFORMANCE H2S |
| 英文摘要 | Semiconducting metal oxides (SMOXs) are used widely for gas sensors. However, the effect of ambient humidity on the baseline and sensitivity of the chemiresistors is still a largely unsolved problem, reducing sensor accuracy and causing complications for sensor calibrations. Presented here is a general strategy to overcome water-sensitivity issues by coating SMOXs with a hydrophobic polymer separated by a metal-organic framework (MOF) layer that preserves the SMOX surface and serves a gas-selective function. Sensor devices using these nanoparticles display near-constant responses even when humidity is varied across a wide range [0-90 % relative humidity (RH)]. Furthermore, the sensor delivers notable performance below 20 % RH whereas other water-resistance strategies typically fail. Selectivity enhancement and humidity-independent sensitivity are concomitantly achieved using this approach. The reported tandem coating strategy is expected to be relevant for a wide range of SMOXs, leading to a new generation of gas sensors with excellent humidity-resistant performance. |
| 源URL | [http://ir.nimte.ac.cn/handle/174433/22189]  |
| 专题 | 中国科学院宁波材料技术与工程研究所 2021专题_期刊论文 |
| 作者单位 | 1.Yang, MH (corresponding author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Peoples R China. 2.Attfield, JP (corresponding author), Univ Edinburgh, Ctr Sci Extreme Condit, Kings Buildings,Mayfield Rd, Edinburgh EH9 3JZ, Midlothian, Scotland. 3.Attfield, JP (corresponding author), Univ Edinburgh, Sch Chem, Kings Buildings,Mayfield Rd, Edinburgh EH9 3JZ, Midlothian, Scotland. |
| 推荐引用方式 GB/T 7714 | Qu, Fengdong,Zhang, Shendan,Huang, Chaozhu,et al. Surface Functionalized Sensors for Humidity-Independent Gas Detection[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2021,60(12):6561-6566. |
| APA | Qu, Fengdong.,Zhang, Shendan.,Huang, Chaozhu.,Guo, Xuyun.,Zhu, Ye.,...&Yang, Minghui.(2021).Surface Functionalized Sensors for Humidity-Independent Gas Detection.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,60(12),6561-6566. |
| MLA | Qu, Fengdong,et al."Surface Functionalized Sensors for Humidity-Independent Gas Detection".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 60.12(2021):6561-6566. |
入库方式： OAI收割
来源：宁波材料技术与工程研究所
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