Enhanced Thermoelectric Properties of p-Type Bi0.48Sb1.52Te3/Sb2Te3 Composite
文献类型:期刊论文
作者 | Shi, Fanfan; Tan, Chang; Wang, Hongxiang; Tan, Xiaojian; Yin, Yinong; Yu, Bo; Cai, Jianfeng; Xiong, Chenglong; Liu, Guoqiang; Jiang, Jun |
刊名 | ACS APPLIED MATERIALS & INTERFACES
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出版日期 | 2020 |
卷号 | 12期号:47页码:52922-52928 |
英文摘要 | Constructing a nanocomposite to introduce a coherent interface is an effective way to improve the property of thermoelectric material. Here, a series composites of Bi0.48Sb1.52Te3-x wt % Sb2Te3 (x = 0, 0.3, 0.5, 0.8, and 1.0) were synthesized, where the hydrothermally prepared Sb2Te3 nanosheets were intimately wrapped in the solid-state-reacted Bi0.48Sb1.52Te3 matrix. The formation of a coherent interface was observed and confirmed by the scanning electron microscopy characterization. As the Sb2Te3 content was over 0.5 wt %, the carrier mobility could increase by 26%, while the carrier concentration decreased by 9% compared to those of the pure matrix at 300 K, enhancing the power factor to 40.1 mu W/cm K-2. Moreover, the Bi0.48Sb1.52Te3-0.5 wt % Sb2Te3 sample exhibited a reduced lattice thermal conductivity of 0.83 W/m K at room temperature, resulting from the strengthened phonon scattering by interfaces. Combined with the manipulations of both the electronic and thermal transport by constructing a coherent interface, a maximum ZT of 1.05 was obtained in the x = 0.5 composite at 300 K, and it was improved by 20% compared with the result of the Bi0.48Sb1.52Te3 matrix. |
源URL | [http://ir.nimte.ac.cn/handle/174433/22440] ![]() |
专题 | 中国科学院宁波材料技术与工程研究所 2020专题_期刊论文 2021专题_期刊论文 |
作者单位 | 1.Yu, B 2.Jiang, J (corresponding author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Peoples R China. 3.Jiang, J (corresponding author), Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China. 4.Tan, XJ |
推荐引用方式 GB/T 7714 | Shi, Fanfan,Tan, Chang,Wang, Hongxiang,et al. Enhanced Thermoelectric Properties of p-Type Bi0.48Sb1.52Te3/Sb2Te3 Composite[J]. ACS APPLIED MATERIALS & INTERFACES,2020,12(47):52922-52928. |
APA | Shi, Fanfan.,Tan, Chang.,Wang, Hongxiang.,Tan, Xiaojian.,Yin, Yinong.,...&Jiang, Jun.(2020).Enhanced Thermoelectric Properties of p-Type Bi0.48Sb1.52Te3/Sb2Te3 Composite.ACS APPLIED MATERIALS & INTERFACES,12(47),52922-52928. |
MLA | Shi, Fanfan,et al."Enhanced Thermoelectric Properties of p-Type Bi0.48Sb1.52Te3/Sb2Te3 Composite".ACS APPLIED MATERIALS & INTERFACES 12.47(2020):52922-52928. |
入库方式: OAI收割
来源:宁波材料技术与工程研究所
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