Photodriven water oxidation initiated by a surface bound chromophore-donor-catalyst assembly
文献类型：期刊论文
| 作者 | Wang, Degao; Xu, Zihao; Sheridan, Matthew V.; Concepcion, Javier J.; Li, Fei; Lian, Tianquan; Meyer, Thomas J. |
| 刊名 | CHEMICAL SCIENCE
 |
| 出版日期 | 2021 |
| 卷号 | 12期号:43页码:14441-14450 |
| 关键词 | INTERFACIAL ELECTRON-TRANSFER OXYGEN-EVOLVING COMPLEX METAL-OXIDE SURFACES ARTIFICIAL PHOTOSYNTHESIS RECOMBINATION DYNAMICS HIGHLY EFFICIENT POLYPYRIDYL DYES PHOTOSYSTEM-II BOND FORMATION SOLAR FUELS |
| 英文摘要 | In photosynthesis, solar energy is used to produce solar fuels in the form of new chemical bonds. A critical step to mimic photosystem II (PS II), a key protein in nature's photosynthesis, for artificial photosynthesis is designing devices for efficient light-driven water oxidation. Here, we describe a single molecular assembly electrode that duplicates the key components of PSII. It consists of a polypyridyl light absorber, chemically linked to an intermediate electron donor, with a molecular-based water oxidation catalyst on a SnO2/TiO2 core/shell electrode. The synthetic device mimics PSII in achieving sustained, light-driven water oxidation catalysis. It highlights the value of the tyrosine-histidine pair in PSII in achieving efficient water oxidation catalysis in artificial photosynthetic devices. |
| 源URL | [http://ir.nimte.ac.cn/handle/174433/21396]  |
| 专题 | 2021专题_期刊论文 |
| 作者单位 | 1.Wang, DG (corresponding author), Chinese Acad Sci, Ningbo Inst Ind Technol, Engn Lab Adv Energy Mat, Ningbo 315201, Zhejiang, Peoples R China. 2.Wang, DG (corresponding author), Qianwan Inst CNiTECH, Zhongchuangyi Rd, Ningbo 315336, Zhejiang, Peoples R China. 3.Wang, DG 4.Meyer, TJ (corresponding author), Univ N Carolina, Dept Chem, Chapel Hill, NC 27599 USA. |
| 推荐引用方式 GB/T 7714 | Wang, Degao,Xu, Zihao,Sheridan, Matthew V.,et al. Photodriven water oxidation initiated by a surface bound chromophore-donor-catalyst assembly[J]. CHEMICAL SCIENCE,2021,12(43):14441-14450. |
| APA | Wang, Degao.,Xu, Zihao.,Sheridan, Matthew V..,Concepcion, Javier J..,Li, Fei.,...&Meyer, Thomas J..(2021).Photodriven water oxidation initiated by a surface bound chromophore-donor-catalyst assembly.CHEMICAL SCIENCE,12(43),14441-14450. |
| MLA | Wang, Degao,et al."Photodriven water oxidation initiated by a surface bound chromophore-donor-catalyst assembly".CHEMICAL SCIENCE 12.43(2021):14441-14450. |
入库方式： OAI收割
来源：宁波材料技术与工程研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。