Covalent triazine frameworks composite membrane (CdS/CTF-1) with enhanced photocatalytic in-situ cleaning and disinfection properties for sustainable separation
文献类型:期刊论文
作者 | Li, Guiliang; Ye, Jianrong; Shen, Yi; Fang, Qile; Liu, Fu |
刊名 | CHEMICAL ENGINEERING JOURNAL
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出版日期 | 2021 |
卷号 | 421 |
关键词 | INTERFACIAL POLYMERIZATION QUANTUM DOTS NANOSHEET OXIDATION |
英文摘要 | Photo-assisted catalysis is proposed to be an effective approach to deal with the membrane fouling issue, which restricts the broad application of burgeoning 2D covalent organic frameworks (COF) membranes in sustainable separation process. In this work, a new type of [0D + 2D] composite membrane was developed via covalent triazine frameworks (CTF-1) nanosheets with built-in CdS quantum dots (QDs). The regular skeleton of 2D-CTF-1 facilitated the uniform growth of CdS QDs (3 nm) on the planar nanosheets. CdS/CTF-1 composite membrane exhibits high water flux (>170 L m- 2 h-1, 0.1 MPa) and high dyes rejection (>94%) via manipulating transportation channels. More importantly, the built-in [0D + 2D]-heterojunction significantly improves the photocatalytic in-situ cleaning and disinfection performance of CdS/CTF-1 membrane, allowing for regenerating permeability (>95%) with the assist of H2O2 during multiple operations. Thus, we provide a prospective strategy to resolve the membrane fouling issues and enable the practical application of 2D membranes for continuous separation. |
源URL | [http://ir.nimte.ac.cn/handle/174433/21448] ![]() |
专题 | 2021专题_期刊论文 |
作者单位 | 1.Liu, F (corresponding author), Chinese Acad Sci, Key Lab Marine Mat & Related Technol, Zhejiang Key Lab Marine Mat & Protect Technol, Ningbo Inst Mat Technol & Engn, 1219 Zhongguan West Rd, Ningbo 315201, Peoples R China. 2.Fang, QL |
推荐引用方式 GB/T 7714 | Li, Guiliang,Ye, Jianrong,Shen, Yi,et al. Covalent triazine frameworks composite membrane (CdS/CTF-1) with enhanced photocatalytic in-situ cleaning and disinfection properties for sustainable separation[J]. CHEMICAL ENGINEERING JOURNAL,2021,421. |
APA | Li, Guiliang,Ye, Jianrong,Shen, Yi,Fang, Qile,&Liu, Fu.(2021).Covalent triazine frameworks composite membrane (CdS/CTF-1) with enhanced photocatalytic in-situ cleaning and disinfection properties for sustainable separation.CHEMICAL ENGINEERING JOURNAL,421. |
MLA | Li, Guiliang,et al."Covalent triazine frameworks composite membrane (CdS/CTF-1) with enhanced photocatalytic in-situ cleaning and disinfection properties for sustainable separation".CHEMICAL ENGINEERING JOURNAL 421(2021). |
入库方式: OAI收割
来源:宁波材料技术与工程研究所
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