Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting
文献类型：期刊论文
| 作者 | Yuan, Cheng-Zong; Hui, Kwan San2; Yin, Hong10; Zhu, Siqi9; Zhang, Jintao8; Wu, Xi-Lin; Hong, Xiaoting6; Zhou, Wei5; Fan, Xi4; Bin F(宾峰)
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| 刊名 | ACS MATERIALS LETTERS
 ; 6
|
| 出版日期 | 2021-07 |
| 卷号 | 3页码:752-780 |
| DOI | 10.1021/acsmaterialslett.0c00549 |
| 英文摘要 | Efficient and low-cost transition-metal (TM)-based electrocatalysts have been of great importance for producing hydrogen (H-2) and oxygen (O-2) via electrocatalytic water (H2O) splitting to ameliorate global energy and environmental problems. However, TM-based materials generally suffer from unsatisfactory electrocatalytic activity because of their relatively low conductivity and unregulated electronic structure. Therefore, the electronic structure engineering of electrocatalysts is an efficient strategic approach to enhance catalytic performances and stabilities. In this review, recent experimental and theoretical advances in the intrinsic electronic structure regulation of TM-based nanomaterials are summarized in terms of preparation methods and underlying natures to boost hydrogen evolution reaction and oxygen evolution reaction. A systematic discussion is conducted on engineering strategies for TM-based nanomaterials to regulate their electronic structures, optimize their adsorption ability of reaction intermediates, and reduce reaction barrier. The existing challenges and perspectives of TM-based electrocatalysts are highlighted to provide new insights into technological advancement for hydrogen production. |
| 学科主题 | Materials Science, Multidisciplinary |
| 分类号 | 一类 |
| 语种 | 英语 |
| WOS记录号 | WOS:000661316200007 |
| 资助机构 | Science and Technology Development Fund, Macau SAR [0191/2017/A3, 0041/2019/A1, 0046/2019/AFJ, 0021/2019/AIR] ; University of Macau [MYRG2017-00216-FST, MYRG2018-00192-IAPME] ; UEA ; Zhejiang Province Basic Public Welfare Research Project [LGF19B070006] ; Science and Technology Program of Guangzhou [2019050001] ; National Key Research and Development Program of China ; Scientific and Technological Plan of Guangdong Province [2018A050506078, 2018B050502010] ; Department of Education of Guangdong Province [2019KZDXM014, 2018KTSCX047] ; China Postdoctoral Science Foundation [2019M662955] ; Natural Science Foundation of Guangdong province [2019A1515011615] ; SCNU Outstanding Young Scholar Project [8S0256] ; UM Macao Postdoctoral Fellowship and Associateship ; Pearl River Talent Program [2019QN01L951] |
| 其他责任者 | Hui, KN (corresponding author), Univ Macau, Inst Appl Phys & Mat Engn, Minist Educ, Joint Key Lab, Taipa 999078, Macau Sar, Peoples R China. ; Hui, KS (corresponding author), Univ East Anglia, Fac Sci, Sch Engn, Norwich NR4 7TJ, Norfolk, England. ; Chen, FM (corresponding author), South China Normal Univ, Sch Phys & Telecommun Engn, State Key Lab Opt Informat Phys & Technol, Guangzhou 510006, Peoples R China. |
| 源URL | [http://dspace.imech.ac.cn/handle/311007/90232]  |
| 专题 | 力学研究所_高温气体动力学国家重点实验室 |
| 作者单位 | 1.Univ East Anglia, Fac Sci, Sch Engn, Norwich NR4 7TJ, Norfolk, England 2.Chinese Acad Sci, Inst Mech, State Key Lab High Temp Gas Dynam, Beijing 100190, Peoples R China 3.Chinese Acad Sci, Ningbo Inst Mat Technol Engn, Ningbo 315201, Peoples R China 4.Xiamen Univ, Dept Mech & Elect Engn, Xiamen 361005, Peoples R China 5.Zhejiang Sci Tech Univ, Dept Chem, Hangzhou 310018, Peoples R China 6.Zhejiang Normal Univ, Coll Geog & Environm Sci, Jinhua 321004, Zhejiang, Peoples R China 7.Shandong Univ, Sch Chem & Chem Engn, Jinan 250061, Peoples R China 8.Anhui Univ Technol, Maanshan, Anhui, Peoples R China 9.Huazhong Univ Sci & Technol, Appl Mat, Wuhan 430074, Hubei, Peoples R China 10.Univ Macau, Inst Appl Phys & Mat Engn, Minist Educ, Joint Key Lab, Taipa 999078, Macau Sar, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yuan, Cheng-Zong,Hui, Kwan San,Yin, Hong,et al. Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting[J]. ACS MATERIALS LETTERS, 6,2021,3:752-780. |
| APA | Yuan, Cheng-Zong.,Hui, Kwan San.,Yin, Hong.,Zhu, Siqi.,Zhang, Jintao.,...&Hui, Kwun Nam.(2021).Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting.ACS MATERIALS LETTERS,3,752-780. |
| MLA | Yuan, Cheng-Zong,et al."Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting".ACS MATERIALS LETTERS 3(2021):752-780. |
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来源：力学研究所
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