Ball-milled magnetite for efficient arsenic decontamination: Insights into oxidation-adsorption mechanism
文献类型：期刊论文
| 作者 | Yang, Xiao7; Liu, Siyan6,7; Liang, Tao6,7; Yan, Xiulan7; Zhang, Yunhui5; Zhou, Yaoyu4; Sarkar, Binoy3; Ok, Yong Sik1,2 |
| 刊名 | JOURNAL OF HAZARDOUS MATERIALS
 |
| 出版日期 | 2022-04-05 |
| 期号 | 427页码:12 |
| 关键词 | Arsenic Magnetite Ball milling Synergistic oxidation Sustainable environmental engineering |
| ISSN号 | 0304-3894 |
| DOI | 10.1016/j.jhazmat.2021.128117 |
| 英文摘要 | Conventional adsorbents for decontaminating arsenic exhibit low efficacy for the removal of arsenite (As (III)). This study aims to develop a robust As adsorbent from natural magnetite (M-0) via a facile ball milling process, and evaluate their performance for decontaminating As(III) and As(V) in water and soil systems. The ball milling process decreased the particle size and crystallinity of M-0, resulting in pronounced As removal by the ball-milled magnetite (M-m). Ball milling under air facilitated the formation of Fe-OH and Fe-COOH functional groups on M-m interface, contributing to effective elimination of As(III) and As(V) via hydrogen bonding and complexation mechanisms. Synergistic oxidation effects of hydroxyl and carboxyl groups, and reactive oxygen species (O-2(-), and center dot OH) on the transformation of As(III) to As(V) during the adsorption were proposed to explain the enhanced As(III) removal by M-m. A short-term soil incubation experiment indicated that the addition of M-m (10 wt%) induced a decrease in the concentration of exchangeable As by 30.25%, and facilitated the transformation of water-soluble As into residual fraction. Ball milling thus is considered as an eco-friendly (chemical-free) and inexpensive (scalable, one-stage process) method for upgrading the performance of natural magnetite towards remediating As, particularly for tackling the highly mobile As(III). |
| WOS关键词 | ZERO-VALENT IRON ; CONTAMINATED SOILS ; NANOPARTICLES ; WATER ; REMOVAL ; EQUILIBRIUM ; BIOCHAR ; OXIDES ; FE3O4 ; LEAD |
| 资助项目 | National Natural Science Foundation of China[U21A2023] ; National Natural Science Foundation of China[U21A2023] ; National Natural Science Foundation of China[41571309] ; National Natural Science Foundation of China[41571309] ; National Research Foundation of Korea (NRF) - Korea government (MSIT)[2021R1A2C2011734] ; National Research Foundation of Korea (NRF) - Korea government (MSIT)[2021R1A2C2011734] ; OJEong Resilience Institute (OJERI) Research Grant from the OJERI, Korea University, Republic of Korea |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000752575300005 |
| 出版者 | ELSEVIER |
| 资助机构 | National Natural Science Foundation of China ; National Research Foundation of Korea (NRF) - Korea government (MSIT) ; OJEong Resilience Institute (OJERI) Research Grant from the OJERI, Korea University, Republic of Korea |
| 源URL | [http://ir.igsnrr.ac.cn/handle/311030/170694]  |
| 专题 | 中国科学院地理科学与资源研究所 |
| 作者单位 | 1.Korea Univ, Div Environm Sci & Ecol Engn, Seoul 02841, South Korea 2.Korea Univ, Korea Biochar Res Ctr, O Jeong Ecoresilience Inst OJERI, Seoul 02841, South Korea 3.Univ Lancaster, Lancaster Environm Ctr, Lancaster LA1 4YQ, England 4.Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China 5.Tongji Univ, Coll Environm Sci & Engn, Shanghai 200092, Peoples R China 6.Univ Chinese Acad Sci, Coll Resources & Environm, Beijing 100190, Peoples R China 7.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Key Lab Land Surface Pattern & Simulat, Beijing 100101, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yang, Xiao,Liu, Siyan,Liang, Tao,et al. Ball-milled magnetite for efficient arsenic decontamination: Insights into oxidation-adsorption mechanism[J]. JOURNAL OF HAZARDOUS MATERIALS,2022(427):12. |
| APA | Yang, Xiao.,Liu, Siyan.,Liang, Tao.,Yan, Xiulan.,Zhang, Yunhui.,...&Ok, Yong Sik.(2022).Ball-milled magnetite for efficient arsenic decontamination: Insights into oxidation-adsorption mechanism.JOURNAL OF HAZARDOUS MATERIALS(427),12. |
| MLA | Yang, Xiao,et al."Ball-milled magnetite for efficient arsenic decontamination: Insights into oxidation-adsorption mechanism".JOURNAL OF HAZARDOUS MATERIALS .427(2022):12. |
入库方式： OAI收割
来源：地理科学与资源研究所
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