Spatial distribution, risk estimation and source apportionment of potentially toxic metal(loid)s in resuspended megacity street dust
文献类型:期刊论文
作者 | Fan, Peng5; Lu, Xinwei5; Yu, Bo5; Fan, Xinyao5; Wang, Lingqing4; Lei, Kai3; Yang, Yufan5; Zuo, Ling5; Rinklebe, Joerg1,2 |
刊名 | ENVIRONMENT INTERNATIONAL
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出版日期 | 2022-02-01 |
卷号 | 160页码:13 |
关键词 | Potentially toxic metal(loid)s Risk assessment Multivariate statistical analysis Positive matrix factorization Resuspended street dust |
ISSN号 | 0160-4120 |
DOI | 10.1016/j.envint.2021.107073 |
英文摘要 | The levels of potentially toxic metal(loid)s (PTMs) As, Cu, Co, Cr, Hg, Mn, Ni, Pb, and Zn in resuspended street dust (<100 mu m particles) from a megacity in north China were determined. The sources of PTMs in resuspended street dust were analyzed using multivariate statistical analysis and positive matrix factorization methods that combined the spatial distributions of PTMs. Average levels of Zn, As, Pb, Cu, Co, and Hg exceeded those found in local soil samples, while those of Cr, Mn, and Ni were less than their background levels found in local soil. The overall contamination of PTMs in resuspended street dust was characterized as moderately contaminated and as uncontaminated to moderately contaminated. The ecological risk associated with Hg was very high, while the ecological risks associated with Cu, Co, Cr, Mn, Ni, Pb, and Zn were low. The overall ecological risk of PTMs was defined as high, driven by Hg. The non-carcinogenic risks of PTMs to inhabitants fell within safety limits, and the carcinogenic risks of As, Co, Cr, and Ni were below receivable values. A comprehensive analysis of PTMs sources revealed that Co, Zn, Cu, and Pb were principally associated with traffic emissions, which accounted for about 38.3% of these PTMs' contents. Mn, Ni, and Cr were mainly generated by natural source, which contributed to about 41.5% of these PTMs' concentrations. Hg and As were primarily derived from coal-related industrial source, which accounted for 77.9% of Hg and 62.9% of As in resuspended street dust. This study demonstrates that coal-related industrial discharges and traffic emissions are the main anthropogenic sources of PTMs contamination in resuspended street dust in the study area. |
WOS关键词 | POLYCYCLIC AROMATIC-HYDROCARBONS ; HEAVY-METALS ; TRACE-ELEMENTS ; ROAD DUST ; URBAN ; CONTAMINATION ; SOILS ; CITY ; PARTICLES ; AREA |
资助项目 | Research and Development Key Project of Shaanxi Province[2020SF-433] ; National Natural Science Foundation of China[41271510] ; Alexander von Humboldt Foundation |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
WOS记录号 | WOS:000760318800009 |
出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
资助机构 | Research and Development Key Project of Shaanxi Province ; National Natural Science Foundation of China ; Alexander von Humboldt Foundation |
源URL | [http://ir.igsnrr.ac.cn/handle/311030/171549] ![]() |
专题 | 陆地表层格局与模拟院重点实验室_外文论文 |
作者单位 | 1.Sejong Univ, Dept Environm, Dept Environm & Energy, Seoul 05006, South Korea 2.Univ Wuppertal, Sch Architecture & Civil Engn, Inst Fdn Engn Water & Waste Management Soil & Gro, Pauluskirchstr 7, D-42285 Wuppertal, Germany 3.Xian Univ, Sch Biol & Environm Engn, Xian 710065, Peoples R China 4.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Key Lab Land Surface Pattern & Simulat, Beijing 100101, Peoples R China 5.Shaanxi Normal Univ, Sch Geog & Tourism, Dept Environm Sci, Xian 710119, Peoples R China |
推荐引用方式 GB/T 7714 | Fan, Peng,Lu, Xinwei,Yu, Bo,et al. Spatial distribution, risk estimation and source apportionment of potentially toxic metal(loid)s in resuspended megacity street dust[J]. ENVIRONMENT INTERNATIONAL,2022,160:13. |
APA | Fan, Peng.,Lu, Xinwei.,Yu, Bo.,Fan, Xinyao.,Wang, Lingqing.,...&Rinklebe, Joerg.(2022).Spatial distribution, risk estimation and source apportionment of potentially toxic metal(loid)s in resuspended megacity street dust.ENVIRONMENT INTERNATIONAL,160,13. |
MLA | Fan, Peng,et al."Spatial distribution, risk estimation and source apportionment of potentially toxic metal(loid)s in resuspended megacity street dust".ENVIRONMENT INTERNATIONAL 160(2022):13. |
入库方式: OAI收割
来源:地理科学与资源研究所
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