中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Source-specific health risks apportionment of soil potential toxicity elements combining multiple receptor models with Monte Carlo simulation

文献类型:期刊论文

作者Lei, Mei1,2; Li, Kai1,2; Guo, Guanghui1,2; Ju, Tienan1,2
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2022-04-15
卷号817页码:15
关键词Soil potential toxicity elements Source apportionment Probabilistic health risk assessment Positive matrix factorization
ISSN号0048-9697
DOI10.1016/j.scitotenv.2021.152899
通讯作者Guo, Guanghui(Guogh@igsnrr.ac.cn)
英文摘要Understanding the source-specific human health risk of soil potential toxicity elements (PTEs) for human is beneficial for pollution control and risk prevention. Multivariate statistics, absolute principal component score/multiple linear regression (APCS/MLR) model, positive matrix factorization (PMF) model, and GIS mapping were used to identify and apportion the sources of soil PTEs in typical mining and industrial area, southwestern China. Furthermore, source-specific health risks were apportioned by combining source apportionment with probabilistic health risk assessment based on Monte Carlo simulation which can define the probability that the risk exceed the guideline threshold value. The pollution factor and geo-accumulation index indicated that the soils were polluted by soil PTEs to different degrees. In particular, As and Cd were the primary pollutants. Mixed sources, agricultural activities, mining activities, and As-related smelting activities represented the potential sources of soil PTEs, with the contribution of 30.13%, 25.78%, 22.93%, and 21.16%, respectively. Source-specific probabilistic health risks indicated that As-related smelting activities contributed the most to non-carcinogenic risks (adults: 59.03%, children: 57.20%) and carcinogenic risks (adults: 81.82%; children 92.33%), despite the observation that it contributed the least to the accumulation of soil PTEs (21.16%). Non-carcinogenic and carcinogenic risk showed similar trend for children and adults. Therefore, Asrelated smelting activities were regarded as the priority source of soil PTEs, and corresponding prevention and control strategies should be implemented to protect human health.
WOS关键词HEAVY-METALS ; AGRICULTURAL SOILS ; SPATIAL-DISTRIBUTION ; INTEGRATED APPROACH ; GUANGDONG PROVINCE ; YUNNAN PROVINCE ; SURFACE SOILS ; CITY ; CONTAMINATION ; ACCUMULATION
资助项目National Key Research and Development Program of China[2018YFC1800104]
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000743200100005
出版者ELSEVIER
资助机构National Key Research and Development Program of China
源URL[http://ir.igsnrr.ac.cn/handle/311030/169825]  
专题中国科学院地理科学与资源研究所
通讯作者Guo, Guanghui
作者单位1.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Lei, Mei,Li, Kai,Guo, Guanghui,et al. Source-specific health risks apportionment of soil potential toxicity elements combining multiple receptor models with Monte Carlo simulation[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2022,817:15.
APA Lei, Mei,Li, Kai,Guo, Guanghui,&Ju, Tienan.(2022).Source-specific health risks apportionment of soil potential toxicity elements combining multiple receptor models with Monte Carlo simulation.SCIENCE OF THE TOTAL ENVIRONMENT,817,15.
MLA Lei, Mei,et al."Source-specific health risks apportionment of soil potential toxicity elements combining multiple receptor models with Monte Carlo simulation".SCIENCE OF THE TOTAL ENVIRONMENT 817(2022):15.

入库方式: OAI收割

来源:地理科学与资源研究所

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