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General Strategies to Construct Highly Efficient Sensing Interfaces for Metal Ions Detection from the Perspective of Catalysis

文献类型：期刊论文

作者Xiao, Xiang-Yu1,4,5; Zhao, Yong-Huan1,4,5; Li, Yong-Yu3; Song, Zong-Yin1,4,5; Chen, Shi-Hua1,4,5; Huang, Hong-Qi2; Yang, Meng4,5; Li, Pei-Hua4,5; Huang, Xing-Jiu4,5
刊名ANALYTICAL CHEMISTRY
出版日期2022-09-23
ISSN号0003-2700
DOI10.1021/acs.analchem.2c01797
通讯作者Yang, Meng(myang@iim.ac.cn) ; Li, Pei-Hua(peihuali@issp.ac.cn) ; Huang, Xing-Jiu(xingjiuhuang@iim.ac.cn)
英文摘要Constructing high-effective electrode sensing interfaces has been considered an effective method for electrochemical detection toward heavy metal ions (HMIs). However, most research has been devoted to enhancing the stripping currents of HMIs by simply improving the adsorptive capacity and conductivity of the electrode modified materials, while lacking theoretical guidelines in fabricating catalytic sensing interfaces. Besides, the understanding of detection mechanisms is quite unscientific from the perspective of catalysis. This perspective summarizes five general strategies in designing highly efficient sensing interfaces in the recent five years, including modulating crystal phases, orientations and planes, defect engineering, ionic valence state cycle engineering, adsorption in situ catalysis strategy, and construction of atomic level catalytic active sites. What's more, the catalytic mechanisms for improving the signals of HMIs, such as boosting the electron transfer rates and conversion rates, lowering the energy barriers, etc., are introduced and emphasized. This study has a great significance in directionally controlling functionalized electrochemical sensors to achieve excellent sensitivity and selectivity in detecting environmental pollutants from the view of catalysis, and it also brings enlightenments and guidance to develop new electroanalytical methods.
WOS关键词SENSITIVE ELECTROCHEMICAL DETECTION ; SINGLE-CRYSTAL FACES ; UNDERPOTENTIAL DEPOSITION ; STRIPPING VOLTAMMETRY ; GOLD NANOCLUSTERS ; HEAVY-METALS ; SURFACE ; PERFORMANCE ; OXIDE ; LEAD
资助项目National Natural Science Foundation of China[21735005] ; National Natural Science Foundation of China[22206187] ; National Natural Science Foundation of China[22204166] ; Presidential Foundation of Hefei Institutes of Physical Science, Chinese Academy of Sciences[YZJJ202102] ; Presidential Foundation of Hefei Institutes of Physical Science, Chinese Academy of Sciences[YZJJ2022QN26] ; Presidential Foundation of Hefei Institutes of Physical Science, Chinese Academy of Sciences[YZJJZX202019] ; China Postdoctoral Innovation Talents Supporting Project[BX2021317] ; Anhui Provincial Natural Science Foundation[2208085QB57]
WOS研究方向Chemistry
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000861194300001
资助机构National Natural Science Foundation of China ; Presidential Foundation of Hefei Institutes of Physical Science, Chinese Academy of Sciences ; China Postdoctoral Innovation Talents Supporting Project ; Anhui Provincial Natural Science Foundation
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/129081]  
专题中国科学院合肥物质科学研究院
通讯作者Yang, Meng; Li, Pei-Hua; Huang, Xing-Jiu
作者单位1.Univ Sci & Technol China, Dept Mat Sci & Engn, Hefei 230026, Peoples R China
2.Anhui Univ, Inst Phys Sci & Informat Technol, Hefei 230601, Peoples R China
3.Tianjin Univ, Sch Environm Sci & Engn, Tianjin 300350, Peoples R China
4.Chinese Acad Sci, Inst Solid State Phys, Environm Mat & Pollut Control Lab, HFIPS, Hefei 230031, Peoples R China
5.Chinese Acad Sci, Inst Solid State Phys, Key Lab Environm Opt & Technol, HFIPS, Hefei 230031, Peoples R China
推荐引用方式
GB/T 7714		 Xiao, Xiang-Yu,Zhao, Yong-Huan,Li, Yong-Yu,et al. General Strategies to Construct Highly Efficient Sensing Interfaces for Metal Ions Detection from the Perspective of Catalysis[J]. ANALYTICAL CHEMISTRY,2022.
APA Xiao, Xiang-Yu.,Zhao, Yong-Huan.,Li, Yong-Yu.,Song, Zong-Yin.,Chen, Shi-Hua.,...&Huang, Xing-Jiu.(2022).General Strategies to Construct Highly Efficient Sensing Interfaces for Metal Ions Detection from the Perspective of Catalysis.ANALYTICAL CHEMISTRY.
MLA Xiao, Xiang-Yu,et al."General Strategies to Construct Highly Efficient Sensing Interfaces for Metal Ions Detection from the Perspective of Catalysis".ANALYTICAL CHEMISTRY (2022).

入库方式： OAI收割

来源：合肥物质科学研究院

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