Al doped Ni-Co layered double hydroxides with surface-sulphuration for highly stable flexible supercapacitors
文献类型:期刊论文
作者 | Wang, Junzeng1; Wang, Zhen1; Liu, Ning1; Liu, Chao1; Yan, Jian1,3,5,6; Li, Chun-Chao4; Cui, Jiewu1; Liu, Jiaqin1,3,5,6; Hu, Xiaoye2; Wu, Yucheng1,2,5,6 |
刊名 | JOURNAL OF COLLOID AND INTERFACE SCIENCE |
出版日期 | 2022-06-01 |
卷号 | 615 |
ISSN号 | 0021-9797 |
关键词 | NiCo-LDH Al doping Surface sulphuration Flexible all-solid-state supercapacitors   PBI solid polymer electrolyte |
DOI | 10.1016/j.jcis.2022.01.172 |
通讯作者 | Yan, Jian(yanjian@hfut.edu.cn) ; Li, Chun-Chao(lcc@mingyangrt.com) ; Hu, Xiaoye(hxy821982@issp.ac.cn) |
英文摘要 | In this work, a strategy of using fast co-precipitation method has been developed to synthesize stable Al doped a-phase NiCo layered double hydroxides (NCA-LDH). A subsequent surface sulphuration of NCA-LDH (S-NCA-LDH) was carried out to improve the conductivity. The as-synthesized S-NCA-LDH exhibits a good electrochemical performance with a specific capacity of 727.1C g(-1) at 1 A g(-1). At 20 A g(-1), the speci-fic capacity still remains 556C g(-1). The capacity retention reaches 95.1 % after 10,000 cycles. Moreover, S-NCA-LDH as positive electrode, activated carbons (AC) as negative electrode and KOH doped polybenzim-idazole (PBI-KOH) as solid polymer electrolyte have been employed to assemble flexible all-solid-state supercapacitors (S-NCA-LDH//PBI-KOH//AC). The device exhibits a specific capacitance of 182.6F g(-1) at 0.5 A g(-1) within 1.8 V. It corresponds to a specific energy of 82.2 Wh kg(-1) at 450 W kg(-1). It also shows a good cycling stability with capacitance retention of about 92.5 % after 10,000 cycles. Further considering the good mechanical performance under bending and folding deformation conditions, the S-NCA-LDH based flexible devices demonstrate the superiority in applications of flexible wearable electronics. (C)& nbsp;2022 Elsevier Inc. All rights reserved. |
WOS关键词 | ASYMMETRIC SUPERCAPACITOR ; GRAPHENE ; PERFORMANCE ; COMPOSITE |
资助项目 | Natural Science Foundation of China[52072104] ; Natural Science Foundation of China[51972093] ; Natural Science Foundation of China[U1910210] ; Natural Science Foundation of China[U1810204] ; Fundamental Research Funds for Central Universities of China[PA2020GDJQ0026] ; Nature Science Research Project of Anhui province[2008085ME129] ; Key Research and Development Plan of Anhui Province[202004b11020024] ; 111 Project[B18018] |
WOS研究方向 | Chemistry |
语种 | 英语 |
出版者 | ACADEMIC PRESS INC ELSEVIER SCIENCE |
WOS记录号 | WOS:000791542400004 |
资助机构 | Natural Science Foundation of China ; Fundamental Research Funds for Central Universities of China ; Nature Science Research Project of Anhui province ; Key Research and Development Plan of Anhui Province ; 111 Project |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/130799] |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Yan, Jian; Li, Chun-Chao; Hu, Xiaoye |
作者单位 | 1.Hefei Univ Technol, Inst Ind & Equipment Technol, Sch Mat Sci & Engn, Hefei 230009, Peoples R China 2.Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Anhui, Peoples R China 3.Key Lab Adv Funct Mat & Devices Anhui Prov, Hefei 230009, Peoples R China 4.Jitoo UHPC Shandong New Mat Technol Co Ltd, Jinan, Shandong, Peoples R China 5.Hefei Univ Technol, China Int S&T Cooperat Base Adv Energy & Environm, Hefei 230009, Peoples R China 6.Hefei Univ Technol, Anhui Prov Int S&T Cooperat Base Adv Energy Mat, Hefei 230009, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Junzeng,Wang, Zhen,Liu, Ning,et al. Al doped Ni-Co layered double hydroxides with surface-sulphuration for highly stable flexible supercapacitors[J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE,2022,615. |
APA | Wang, Junzeng.,Wang, Zhen.,Liu, Ning.,Liu, Chao.,Yan, Jian.,...&Wu, Yucheng.(2022).Al doped Ni-Co layered double hydroxides with surface-sulphuration for highly stable flexible supercapacitors.JOURNAL OF COLLOID AND INTERFACE SCIENCE,615. |
MLA | Wang, Junzeng,et al."Al doped Ni-Co layered double hydroxides with surface-sulphuration for highly stable flexible supercapacitors".JOURNAL OF COLLOID AND INTERFACE SCIENCE 615(2022). |
入库方式: OAI收割
来源:合肥物质科学研究院
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