中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Spectral broadening mechanism of Yb3+-doped cubic LuxSc2-xO3 sesquioxide crystals for ultrafast lasers

文献类型:期刊论文

作者Guo, Ruiqi2,3; Huang, Dapeng2,3; Lu, Dazhi2,3; Liang, Fei2,3; Zhang, Qingli1; Yu, Haohai2,3; Zhang, Huaijin2,3
刊名OPTICAL MATERIALS EXPRESS
出版日期2022-05-01
卷号12
ISSN号2159-3930
DOI10.1364/OME.451476
通讯作者Lu, Dazhi(dazhi.lu@sdu.edu.cn)
英文摘要Over the past decades, Yb3+-doped cubic sesquioxide crystals have been considered as ideal gain materials for ultrafast laser generation, owing to their high thermal conductivity and adequate optical characteristics. The broadening of spectra by mixing host crystals to obtain short pulses has been extensively explored; however, few studies have examined the mechanism of the crystal field effect on spectral broadening. This paper describes the spectral broadening process caused by the combination of the discrete transition peaks induced by the crystal field effect and electron-phonon coupling widening based on Yb:LuxSc2-xO3 crystals. The energy level splitting induced by the crystal field effect not only determines the emission peak positions, but also broadens the emission spectra in the mixed host materials through the increasing spin-orbit coupling effect. Moreover, with the involvement of the electron-phonon coupling and the crystal field effect, the spectral broadening is much more obvious at room temperature. These results not only explain the spectral broadening mechanism of Yb3+-doped sesquioxides but also provide important insights for the improvement of new ultrafast laser materials. (C) 2022 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement
WOS关键词EFFECTIVE IONIC-RADII ; FIELD PARAMETERS ; DIODE ; GENERATION ; PULSES ; MODEL
资助项目National Key Research and Development Program of China[2016YFB1102301] ; National Natural Science Foundation of China[51772173] ; National Natural Science Foundation of China[51802307] ; National Natural Science Foundation of China[51902181] ; National Natural Science Foundation of China[52025021]
WOS研究方向Materials Science ; Optics
语种英语
WOS记录号WOS:000799154500002
出版者Optica Publishing Group
资助机构National Key Research and Development Program of China ; National Natural Science Foundation of China
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/131069]  
专题中国科学院合肥物质科学研究院
通讯作者Lu, Dazhi
作者单位1.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Hefei 230031, Peoples R China
2.Shandong Univ, State Key Lab Crystal Mat, Jinan 250100, Peoples R China
3.Shandong Univ, Inst Crystal Mat, Jinan 250100, Peoples R China
推荐引用方式
GB/T 7714
Guo, Ruiqi,Huang, Dapeng,Lu, Dazhi,et al. Spectral broadening mechanism of Yb3+-doped cubic LuxSc2-xO3 sesquioxide crystals for ultrafast lasers[J]. OPTICAL MATERIALS EXPRESS,2022,12.
APA Guo, Ruiqi.,Huang, Dapeng.,Lu, Dazhi.,Liang, Fei.,Zhang, Qingli.,...&Zhang, Huaijin.(2022).Spectral broadening mechanism of Yb3+-doped cubic LuxSc2-xO3 sesquioxide crystals for ultrafast lasers.OPTICAL MATERIALS EXPRESS,12.
MLA Guo, Ruiqi,et al."Spectral broadening mechanism of Yb3+-doped cubic LuxSc2-xO3 sesquioxide crystals for ultrafast lasers".OPTICAL MATERIALS EXPRESS 12(2022).

入库方式: OAI收割

来源:合肥物质科学研究院

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