Electrocatalytic Reduction of Nitrogen to Ammonia in Ionic Liquids br
文献类型:期刊论文
作者 | Tian, Yuan1,2; Liu, Yanrong2,3; Wang, Hao2; Liu, Lei2,4; Hu, Wenping1 |
刊名 | ACS SUSTAINABLE CHEMISTRY & ENGINEERING
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出版日期 | 2022-04-11 |
卷号 | 10期号:14页码:4345-4358 |
关键词 | Ammonia synthesis Electrocatalysis Nitrogen reduction reaction Ionic liquids Electrocatalytic NRR process Ambient conditions |
ISSN号 | 2168-0485 |
DOI | 10.1021/acssuschemeng.2c00018 |
英文摘要 | Ammonia (NH3) is an important raw material fornitrogen fertilizer production and is widely used in industry. It is alsoa carbon-free renewable fuel and an excellent hydrogen storagematerial. Reaction conditions of the traditional Haber-Bosch processare very harsh even though it supports most of today'sNH3production. Recently, the electrocatalytic nitrogen reduction reaction(NRR) has become one of the effective alternative methods to thetraditional Haber-Bosch process due to the advantages of mildoperation conditions and almost no environmental pollution. Ionicliquids (ILs) act as one of the green solvents that possess a lot ofunique features and have shown excellent performance in theelectrocatalytic NRR process. In this perspective, we summarize thefundamentals of the electrocatalytic NRR, the role of ILs in severaltypical electrocatalytic processes, and the possible role of ILs in theelectrocatalytic NRR process. Moreover, the selection principles and issues of the application of ILs as well as the futuredevelopment directions for the electrocatalytic NRR process are presented. |
WOS关键词 | ELECTROCHEMICAL REDUCTION ; OXYGEN-REDUCTION ; PHYSICOCHEMICAL PROPERTIES ; CARBON-DIOXIDE ; CO2 REDUCTION ; CATALYSTS ; N-2 ; SOLUBILITY ; DINITROGEN ; CONVERSION |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Engineering |
语种 | 英语 |
WOS记录号 | WOS:000791025300002 |
出版者 | AMER CHEMICAL SOC |
源URL | [http://ir.ipe.ac.cn/handle/122111/53347] ![]() |
专题 | 中国科学院过程工程研究所 |
通讯作者 | Liu, Lei; Hu, Wenping |
作者单位 | 1.Tianjin Univ, Sch Sci, Dept Chem, Tianjin Key Lab Mol Optoelect Sci, Tianjin 300072, Peoples R China 2.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, CAS Key Lab Green Proc & Engn, State Key Lab Multiphase Complex Syst,Inst Proc E, Beijing 100190, Peoples R China 3.Zhengzhou Inst Emerging Ind Technol, Zhengzhou 450000, Peoples R China 4.Wuhan Text Univ, Sch Chem & Chem Engn, Wuhan 430200, Peoples R China |
推荐引用方式 GB/T 7714 | Tian, Yuan,Liu, Yanrong,Wang, Hao,et al. Electrocatalytic Reduction of Nitrogen to Ammonia in Ionic Liquids br[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2022,10(14):4345-4358. |
APA | Tian, Yuan,Liu, Yanrong,Wang, Hao,Liu, Lei,&Hu, Wenping.(2022).Electrocatalytic Reduction of Nitrogen to Ammonia in Ionic Liquids br.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,10(14),4345-4358. |
MLA | Tian, Yuan,et al."Electrocatalytic Reduction of Nitrogen to Ammonia in Ionic Liquids br".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 10.14(2022):4345-4358. |
入库方式: OAI收割
来源:过程工程研究所
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