CFD simulation of an industrial MTO fluidized bed by coupling a population balance model of coke content
文献类型：期刊论文
| 作者 | Zhang, Chunhua2,3; Lu, Bona1,2; Wang, Wei1,2 ; Liu, Mengxi3; Lu, Chunxi3; Ye, Mao4
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| 刊名 | CHEMICAL ENGINEERING JOURNAL
 |
| 出版日期 | 2022-10-15 |
| 卷号 | 446页码:10 |
| 关键词 | MTO PBM CFD Fluidization Mesoscale Modeling |
| ISSN号 | 1385-8947 |
| DOI | 10.1016/j.cej.2022.136849 |
| 英文摘要 | The coke distribution over shape-selective catalysts in fluidized bed reactors is critical to the selectivity of target products. A population balance model (PBM) is developed in this study to describe the evolution of coke distribution due to both reactions and circulation of catalysts. The PBM is coupled with multiscale computational fluid dynamics (CFD) to simulate a methanol-to-olefins fluidized bed reactor. A wide, uneven distribution of coke content can thus be predicted. The mass fractions of the desired products, ethylene and propylene, show better agreement with the experimental data than those without PBM. And the selectivity ratio of ethylene to propylene is also better predicted. Furthermore, the relaxation time of fresh catalyst is considered to express the effects of the induction period in MTO reactions. The reasonable prediction suggests that coupling PBM with multiscale CFD is helpful to understand MTO reactors and may find more application with respect to its optimization and scale-up. |
| WOS关键词 | MULTISCALE CFD ; NUMERICAL-SIMULATION ; METHANOL CONVERSION ; REACTION BEHAVIORS ; SOLID FLOW ; OLEFINS ; REACTOR ; POLYMERIZATION ; DEACTIVATION ; GROWTH |
| 资助项目 | National Natural Science Foundation of China[91834302] ; National Natural Science Foundation of China[22078331] ; National Natural Science Foundation of China[22161142006] ; State Key Laboratory of Multiphase Complex Systems of China[MPCS-2021-D-05] ; National Science and Technology Major Project[2017-I-0004-0005] ; Transformational Technologies for Clean Engery and Demonstration?[XDA21030700] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA21030700] |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000803700100004 |
| 出版者 | ELSEVIER SCIENCE SA |
| 资助机构 | National Natural Science Foundation of China ; State Key Laboratory of Multiphase Complex Systems of China ; National Science and Technology Major Project ; Transformational Technologies for Clean Engery and Demonstration? ; Strategic Priority Research Program of the Chinese Academy of Sciences |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/53478]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Lu, Bona; Wang, Wei; Lu, Chunxi |
| 作者单位 | 1.Univ Chinese Acad Sci, Sch Chem Engn, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 3.China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China 4.Chinese Acad Sci, Dalian Inst Chem Phys, Natl Engn Lab MTO, Dalian 116023, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Chunhua,Lu, Bona,Wang, Wei,et al. CFD simulation of an industrial MTO fluidized bed by coupling a population balance model of coke content[J]. CHEMICAL ENGINEERING JOURNAL,2022,446:10. |
| APA | Zhang, Chunhua,Lu, Bona,Wang, Wei,Liu, Mengxi,Lu, Chunxi,&Ye, Mao.(2022).CFD simulation of an industrial MTO fluidized bed by coupling a population balance model of coke content.CHEMICAL ENGINEERING JOURNAL,446,10. |
| MLA | Zhang, Chunhua,et al."CFD simulation of an industrial MTO fluidized bed by coupling a population balance model of coke content".CHEMICAL ENGINEERING JOURNAL 446(2022):10. |
入库方式： OAI收割
来源：过程工程研究所
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