Enhancing interface compatibility of UiO-66-NH2 and polyamide by incorporating dopamine into thin film nanocomposite membranes
文献类型：期刊论文
| 作者 | Chen, Long1; Ren, Xiaomin1; Li, Yanxiang2; Hu, Dan1; Feng, Xudong1; Li, Wangliang2 |
| 刊名 | JOURNAL OF MEMBRANE SCIENCE
 |
| 出版日期 | 2022-07-15 |
| 卷号 | 654页码:11 |
| ISSN号 | 0376-7388 |
| 关键词 | Dopamine Interfacial polymerization TFN Ionic selectivity UiO-66-NH2 |
| DOI | 10.1016/j.memsci.2022.120565 |
| 英文摘要 | The introduction of nanoparticles into nanofiltration (NF) membranes is an effective approach to improve the NF performance as the construction of water channels in the nanoparticles. However, the poor compatibility be-tween polymer matrix and nanoparticles is a crucial issue that attracts numerous researchers. In this paper, dopamine (DA) molecule was introduced into the aqueous solution for preparing NF membranes by interfacial polymerization to build a bridge between polyamide matrix and nanoparticles (polydopamine coated UiO-66-NH2, U@PD) for its self-polymerization and high reactive activity of abundant of hydroxyl and amino groups. It was found that the addition of DA in aqueous reaction phase solution effectively reduced the membrane surface roughness, anchored more U@PD nanoparticles, improved the hydrophilicity of the membrane, and participated in the interfacial polymerization reaction to crosslink the nanoparticles and the polyamide matrix. The DA introduced TFN membrane achieved high water permeance (13.87 L.m(-2).h(-1).bar(-1)) and Na2SO4 rejection (97.96%) with DA concentration of 0.3 g/L, U@PD incorporating amount of 0.3 wt%, cross-linking reaction time of 45 min, and pH of 8.5. Additionally, the as-prepared membrane had an excellent selectivity of Cl-/SO42-(alpha = 45.85), which was higher than that of the membrane without DA crosslinking agent (alpha = 14.40). It is concluded that the addition of DA in the interfacial polymerization aqueous solution can effectively repair the defects between the nanoparticles and the polymer, thus provide a new idea for seawater desalination. |
| WOS关键词 | HOLLOW-FIBER MEMBRANES ; LOOSE NANOFILTRATION MEMBRANE ; HIGH-FLUX ; SURFACE MODIFICATION ; GRAPHENE OXIDE ; POLYDOPAMINE ; COMPOSITE ; SEPARATION ; FABRICATION ; EFFICIENT |
| 资助项目 | Scientific Technological Innovation Service Ability Construction-Basic Scientific Research Funding[PXM2020_014213_000017] ; Open Research Fund Program of Key Laboratory of Cleaner Production and Integrated Resource Utilization of China National Light Industry[CP-2020YB4] ; Research Foundation for Youth Scholars of Beijing Technology and Business University[QNJJ2020-18] ; Postgraduate Research Ability Enhancement Project[19008020144] ; Postgraduate Research Ability Enhancement Project[19008021082] |
| WOS研究方向 | Engineering ; Polymer Science |
| 语种 | 英语 |
| 出版者 | ELSEVIER |
| WOS记录号 | WOS:000797883200001 |
| 资助机构 | Scientific Technological Innovation Service Ability Construction-Basic Scientific Research Funding ; Open Research Fund Program of Key Laboratory of Cleaner Production and Integrated Resource Utilization of China National Light Industry ; Research Foundation for Youth Scholars of Beijing Technology and Business University ; Postgraduate Research Ability Enhancement Project |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/53525]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Hu, Dan; Feng, Xudong; Li, Wangliang |
| 作者单位 | 1.Beijing Technol & Business Univ, Sch Light Ind, Key Lab Cleaner Prod & Integrated Resource Utiliza, China Natl Light Ind, Beijing 100048, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, CAS Key Lab Green Proc & Engn, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Long,Ren, Xiaomin,Li, Yanxiang,et al. Enhancing interface compatibility of UiO-66-NH2 and polyamide by incorporating dopamine into thin film nanocomposite membranes[J]. JOURNAL OF MEMBRANE SCIENCE,2022,654:11. |
| APA | Chen, Long,Ren, Xiaomin,Li, Yanxiang,Hu, Dan,Feng, Xudong,&Li, Wangliang.(2022).Enhancing interface compatibility of UiO-66-NH2 and polyamide by incorporating dopamine into thin film nanocomposite membranes.JOURNAL OF MEMBRANE SCIENCE,654,11. |
| MLA | Chen, Long,et al."Enhancing interface compatibility of UiO-66-NH2 and polyamide by incorporating dopamine into thin film nanocomposite membranes".JOURNAL OF MEMBRANE SCIENCE 654(2022):11. |
入库方式： OAI收割
来源：过程工程研究所
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