Recent progress in sustainable recycling of LiFePO4-type lithium-ion batteries: Strategies for highly selective lithium recovery
文献类型：期刊论文
| 作者 | Kumar, Jai3,4; Neiber, Rana R.5,6; Park, Jaewon3; Soomro, Razium Ali4; Greene, George W.7,8; Mazari, Shaukat Ali9; Seo, Heun Young1; Lee, Jin Hong10; Shon, Minyoung2,3; Chang, Dong Wook2,3 |
| 刊名 | CHEMICAL ENGINEERING JOURNAL
 |
| 出版日期 | 2022-03-01 |
| 卷号 | 431页码:16 |
| 关键词 | Selective recycling Sustainable recovery Hazards Spent-batteries Lithium extraction Spent LiFePO4 cathode |
| ISSN号 | 1385-8947 |
| DOI | 10.1016/j.cej.2021.133993 |
| 英文摘要 | The demand for LiFePO4 (LFP)-type batteries have increased remarkably in energy storage devices due to a longer life span, improved discharge and charge efficiency, and safe handling. The growing use of such batteries has raised concern about their proper disposal, where improper handling might result in hazardous material entering the environment. As a result, waste LFP battery recycling is receiving a lot of attention. To date, the recycling of spent LFP batteries has been carried with two traditional methods: (1) pyrometallurgy (i.e., direct regeneration) and (2) hydrometallurgy (i.e., the leaching of individual metals). However, the toxic off-gassing at high temperatures were eventually found not in favor of the environment. Besides, hydrometallurgical recovery of complete metal ions (i.e., Li, Fe, and P) in solution increases the cost of the process due to excess use of minerals. To this end, a hydrometallurgical derived process commonly known as one-step selective recovery of Li and FePO4 are keenly focused, where in-situ recovery of Li in leaching solution and Fe as FePO4 in residue are followed. This review is directed to the selective recovery of Li from the spent LFP cathode materials. The discussion centers on the present process of selective recovery in comparison to the traditional approaches. The structure of LFP and Li-recovery routes, which involve various kinds of leaching agents, are discussed. The effective separation procedures and their advancement are examined, which may pave the way for new and updated technologies to increase environmentally friendly recycling routes. Finally, endeavors are given to the challenges and future aspects of recycling LFP cathode materials. In general, the review will aid in understanding the evolution of a sustainable Li-ion battery recycling methods. |
| WOS关键词 | IRON PHOSPHATE BATTERIES ; POSITIVE-ELECTRODE MATERIALS ; CATHODE MATERIALS ; SPENT LIFEPO4 ; PERFORMANCE ; LI ; FUTURE ; WASTE ; REGENERATION ; METALS |
| 资助项目 | National Research Foundation of Korea (NRF) - Korean government (MSIP)[2021R1F1A1045518] ; National R&D Program through the National Research Foundation of Korea (NRF) - Ministry of Science and ICT[2020M3H4A3106356] |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000799586200006 |
| 出版者 | ELSEVIER SCIENCE SA |
| 资助机构 | National Research Foundation of Korea (NRF) - Korean government (MSIP) ; National R&D Program through the National Research Foundation of Korea (NRF) - Ministry of Science and ICT |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/53628]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Cho, Kie Yong |
| 作者单位 | 1.Korea Univ, Dept Mat Sci & Engn, 145 Anam Ro, Seoul 136713, South Korea 2.Pukyong Natl Univ, Div Appl Chem Engn, Pusan 48547, South Korea 3.Pukyong Natl Univ, Dept Ind Chem, 45 Yongso Ro, Busan 48513, South Korea 4.Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing Key Lab Electrochem Proc & Technol Mat, Beijing 100029, Peoples R China 5.Univ Chinese Acad Sci, Coll Chem Engn, 19 A Yuquan Rd, Beijing 100049, Peoples R China 6.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, CAS Key Lab Green Proc & Engn, Inst Proc Engn, Beijing, Peoples R China 7.Deakin Univ, Inst Frontier Mat, 221 Burwood Highway, Melbourne, Vic 3216, Australia 8.Deakin Univ, ARC Ctr Excellence Electromateriols Sci, 221 Burwood Highway, Melbourne, Vic 3216, Australia 9.Dawood Univ Engn & Technol, Dept Chem Engn, Karachi 74800, Pakistan 10.Pusan Natl Univ, Sch Chem Engn, Busan 46421, South Korea |
| 推荐引用方式 GB/T 7714 | Kumar, Jai,Neiber, Rana R.,Park, Jaewon,et al. Recent progress in sustainable recycling of LiFePO4-type lithium-ion batteries: Strategies for highly selective lithium recovery[J]. CHEMICAL ENGINEERING JOURNAL,2022,431:16. |
| APA | Kumar, Jai.,Neiber, Rana R..,Park, Jaewon.,Soomro, Razium Ali.,Greene, George W..,...&Cho, Kie Yong.(2022).Recent progress in sustainable recycling of LiFePO4-type lithium-ion batteries: Strategies for highly selective lithium recovery.CHEMICAL ENGINEERING JOURNAL,431,16. |
| MLA | Kumar, Jai,et al."Recent progress in sustainable recycling of LiFePO4-type lithium-ion batteries: Strategies for highly selective lithium recovery".CHEMICAL ENGINEERING JOURNAL 431(2022):16. |
入库方式： OAI收割
来源：过程工程研究所
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