A dual regulation strategy for MXene-based composite membrane to achieve photocatalytic self-cleaning properties and multi-functional applications
文献类型：期刊论文
| 作者 | Lin, Qingquan2,3; Zeng, Guangyong1,2,3; Pu, Shengyan2; Yan, Guilong3; Luo, Jianquan1; Wan, Yinhua1; Zhao, Ziyan4 |
| 刊名 | CHEMICAL ENGINEERING JOURNAL
 |
| 出版日期 | 2022-09-01 |
| 卷号 | 443页码:13 |
| ISSN号 | 1385-8947 |
| 关键词 | Dual regulation MXene nanosheets Photocatalytic membrane Self-cleaning mechanism Multi-functional applications |
| DOI | 10.1016/j.cej.2022.136335 |
| 英文摘要 | The development of two-dimensional (2D) membrane materials is limited by their relatively low antifouling performance. The high oxidation activity of photocatalytic technology can degrade the contaminants depositing on the membrane, which is expected to solve the problem of membrane fouling. Here, we reported a dual regulation strategy to construct a composite membrane, including chitosan modified MXene nanosheets as separation layer as well as g-C3N4 photocatalyst blended PVDF membrane as support layer. Scanning electron microscopy (SEM), X-ray photoelectron spectroscopy (XPS) and atomic force microscopy (AFM) are used to verify the successful preparation of the dual interface composite membrane. Experimental results showed that the novel composite membrane exhibited high water permeability as well as achieved excellent rejection of anionic dyes and heavy metal ions (Congo red: over 98 % and Cr6+: 85.4%). Owing to photocatalytic activity, the composite membrane almost completely removed rhodamine B and tetracycline hydrochloride, and its selfcleaning ability improved the anti-fouling performance. Based on density functional theory, we further confirmed that the strong photocatalytic activity of the composite membrane was attributed to the efficient charge transfer between the photocatalytic support layer and the MXene separation layer. This work not only deepened the study of 2D-based materials in membrane preparation, but also provided a new dual regulation strategy to enhance multi-pollutants removal by composite membranes in wastewater treatment. |
| WOS关键词 | GRAPHITIC CARBON NITRIDE ; G-C3N4 ; WATER ; EFFICIENT ; REMOVAL |
| 资助项目 | National Key Research and Development Program of China[2020YFC1808300] ; National Natural Science Foundation of China[42077185] ; Applied Basic Research Programs of Science and Technology Commis-sion Foundation of Sichuan Province[2021YJ0401] |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| 出版者 | ELSEVIER SCIENCE SA |
| WOS记录号 | WOS:000799614900003 |
| 资助机构 | National Key Research and Development Program of China ; National Natural Science Foundation of China ; Applied Basic Research Programs of Science and Technology Commis-sion Foundation of Sichuan Province |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/53675]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Zeng, Guangyong; Luo, Jianquan |
| 作者单位 | 1.Univ Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China 2.Chengdu Univ Technol, State Key Lab Geohazard Prevent & Geoenvironm Prot, Chengdu 610059, Sichuan, Peoples R China 3.Chengdu Univ Technol, Coll Mat & Chem & Chem Engn, Chengdu 610059, Sichuan, Peoples R China 4.Chengdu Qinhuan Technol Co Ltd, Chengdu 610000, Sichuan, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lin, Qingquan,Zeng, Guangyong,Pu, Shengyan,et al. A dual regulation strategy for MXene-based composite membrane to achieve photocatalytic self-cleaning properties and multi-functional applications[J]. CHEMICAL ENGINEERING JOURNAL,2022,443:13. |
| APA | Lin, Qingquan.,Zeng, Guangyong.,Pu, Shengyan.,Yan, Guilong.,Luo, Jianquan.,...&Zhao, Ziyan.(2022).A dual regulation strategy for MXene-based composite membrane to achieve photocatalytic self-cleaning properties and multi-functional applications.CHEMICAL ENGINEERING JOURNAL,443,13. |
| MLA | Lin, Qingquan,et al."A dual regulation strategy for MXene-based composite membrane to achieve photocatalytic self-cleaning properties and multi-functional applications".CHEMICAL ENGINEERING JOURNAL 443(2022):13. |
入库方式： OAI收割
来源：过程工程研究所
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