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The novel 2-dimensional Bi2MoO6-Bi2O3-Ag3PO4 ternary photocatalyst with n-n-p heterojunction for enhanced degradation performance

文献类型:期刊论文

作者Sun, Kaiyue1; Zhou, Hualei1; Li, Xinyang1; Ma, Xiaohui1; Zhang, Donghai2; Li, Mengchao1
刊名JOURNAL OF ALLOYS AND COMPOUNDS
出版日期2022-08-25
卷号913页码:11
关键词Photocatalysis Bi2MoO6 Bi2O3 Ag3PO4 Heterojunction Tetracycline
ISSN号0925-8388
DOI10.1016/j.jallcom.2022.165119
英文摘要The ternary Bi2MoO6-Bi2O3-Ag3PO4 photocatalysts were fabricated via hydrothermal and precipitation methods. Various characterizations proved that the Bi2O3 nanodots and spherical Ag(3)PO(4 )particles were embedded on Bi2MoO6 nanoflakes to form the ternary heterojunction. Compared to single Bi2O3, Bi2MoO6 and the binary Bi2MoO6-Bi2O3, the ternary composites at optimum Ag3PO4 content possess a significantly high visible-light degradation rate of tetracycline which is 3.2, 4.3 and 1.9 fold that of Bi2MoO6, Bi2O3 and Bi2MoO6-Bi2O3, respectively. The enhanced photocatalytic performance is attributed to the formation of ternary heterojunction that could greatly promote the transfer and separation of photo-generated carriers and extend the visible-light response range. The superoxide radical (center dot O-2(-)) played a key role in the photo catalytic process and the photocatalytic mechanism of the ternary n-n-p heterojunctions were proposed. This work could offer a new insight in manufacturing ternary photocatalysts for the degradation of tetracycline under visible light irradiation. (C) 2022 Elsevier B.V. All rights reserved.
WOS关键词Z-SCHEME PHOTOCATALYST ; HYDROGEN EVOLUTION ; HIGHLY EFFICIENT ; BI2MOO6 ; FABRICATION ; MECHANISM ; COMPOSITES ; ABSORPTION ; SOLAR
资助项目Open Research Fund of State Key Laboratory of Multiphase Complex Systems of China[MPCS-2021-D-11]
WOS研究方向Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering
语种英语
WOS记录号WOS:000804647400001
出版者ELSEVIER SCIENCE SA
资助机构Open Research Fund of State Key Laboratory of Multiphase Complex Systems of China
源URL[http://ir.ipe.ac.cn/handle/122111/53730]  
专题中国科学院过程工程研究所
通讯作者Zhou, Hualei
作者单位1.Univ Sci & Technol Beijing, Dept Chem & Chem Engn, Beijing Key Lab Sci & Applicat Funct Mol & Crystal, Beijing 100083, Peoples R China
2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Sun, Kaiyue,Zhou, Hualei,Li, Xinyang,et al. The novel 2-dimensional Bi2MoO6-Bi2O3-Ag3PO4 ternary photocatalyst with n-n-p heterojunction for enhanced degradation performance[J]. JOURNAL OF ALLOYS AND COMPOUNDS,2022,913:11.
APA Sun, Kaiyue,Zhou, Hualei,Li, Xinyang,Ma, Xiaohui,Zhang, Donghai,&Li, Mengchao.(2022).The novel 2-dimensional Bi2MoO6-Bi2O3-Ag3PO4 ternary photocatalyst with n-n-p heterojunction for enhanced degradation performance.JOURNAL OF ALLOYS AND COMPOUNDS,913,11.
MLA Sun, Kaiyue,et al."The novel 2-dimensional Bi2MoO6-Bi2O3-Ag3PO4 ternary photocatalyst with n-n-p heterojunction for enhanced degradation performance".JOURNAL OF ALLOYS AND COMPOUNDS 913(2022):11.

入库方式: OAI收割

来源:过程工程研究所

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