Rational design of 3D net-like carbon based Mn3O4 anode materials with enhanced lithium storage performance
文献类型：期刊论文
| 作者 | Li, Xue2; Yue, Wence2; Li, Wenbiao2; Zhao, Jie2; Zhang, Yujiao2; Gao, Yibo2; Gao, Ning2; Feng, Dan2; Wu, Bin1,3; Wang, Bao2,4 |
| 刊名 | NEW JOURNAL OF CHEMISTRY
 |
| 出版日期 | 2022-06-09 |
| 页码 | 8 |
| ISSN号 | 1144-0546 |
| DOI | 10.1039/d2nj01618d |
| 英文摘要 | An optimized structure design of three-dimensional (3D) net-like carbon based Mn3O4 (Mn3O4/CP) composites was realized based on the theory of explosive nucleation and in situ growth. Mn3O4/CP composites have been successfully prepared on a large scale with filter paper adsorbed with manganese(ii) oleate as the raw materials using a facile thermal decomposition route. The obtained Mn3O4/CP composite shows a reversible capacity of 1005 mA h g(-1) after 90 cycles at a current density of 100 mA g(-1), with a remarkably enhanced rate performance and excellent cycling stability compared to the pure Mn3O4 nanostructure which loses most of its capacity within 10 cycles. Even at a current density of 2000 mA g(-1), the specific capacity of the Mn3O4/CP composite was still as high as 486 mA h g(-1), which is much higher than that of pure Mn3O4 (38 mA h g(-1)) and the carbon materials (111 mA h g(-1)). The enhancement of the electrochemical performance could be attributed to the synergy of Mn3O4 enwrapped with the 3D conductive carbon network, thus making it a promising anode material for large-scale energy storage applications. Moreover, this facile and effective synthetic strategy can be further explored as a universal approach for the rapid synthesis of other transition metal oxides and carbon hybrids with subtle structure engineering. |
| WOS关键词 | HIGH-CAPACITY ; ELECTROCHEMICAL PROPERTIES ; HYDROTHERMAL SYNTHESIS ; ION BATTERY ; MN3O4/GRAPHENE COMPOSITES ; GENERAL-SYNTHESIS ; FACILE SYNTHESIS ; GRAPHENE SHEETS ; HYBRID ; NANOTUBES |
| 资助项目 | National Natural Science Foundation of China[51772296] ; National Natural Science Foundation of China[5217020858] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000815170200001 |
| 出版者 | ROYAL SOC CHEMISTRY |
| 资助机构 | National Natural Science Foundation of China |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/53999]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Wu, Bin; Wang, Bao |
| 作者单位 | 1.Humboldt Univ, Inst Phys, Newton Str 15, D-12489 Berlin, Germany 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China 3.Helmholtz Zentrum Berlin Mat & Energie GmbH, Young Investigator Grp Nanoscale Solid Liquid Int, Albert Einstein Str 15, D-12489 Berlin, Germany 4.Univ Chinese Acad Sci, Coll Chem & Chem Engn, Beijing 100000, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Xue,Yue, Wence,Li, Wenbiao,et al. Rational design of 3D net-like carbon based Mn3O4 anode materials with enhanced lithium storage performance[J]. NEW JOURNAL OF CHEMISTRY,2022:8. |
| APA | Li, Xue.,Yue, Wence.,Li, Wenbiao.,Zhao, Jie.,Zhang, Yujiao.,...&Wang, Bao.(2022).Rational design of 3D net-like carbon based Mn3O4 anode materials with enhanced lithium storage performance.NEW JOURNAL OF CHEMISTRY,8. |
| MLA | Li, Xue,et al."Rational design of 3D net-like carbon based Mn3O4 anode materials with enhanced lithium storage performance".NEW JOURNAL OF CHEMISTRY (2022):8. |
入库方式： OAI收割
来源：过程工程研究所
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