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Progress of the Structure-property Correlation of Heteroatomic Coordination Structured Carbon-based Single-atom Electrocatalysts

文献类型：期刊论文

作者XIA Tian2,3; WAN Jiawei1,3; YU Ranbo2
刊名CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE
出版日期2022-05-10
卷号43期号:5页码:21
ISSN号0251-0790
关键词Heteroatomic coordination structure Single-atom-catalyst Electrocatalysis Electronic structure Mass transfer
DOI10.7503/cjcu20220162
英文摘要Single-atom catalysts are a class of supported catalysts with high atomic economy and high activity using mutually isolated single metal atoms as the catalytic active center,which have been widely used in energy electroca-talysis. In recent years,researchers have constructed single-atom electrocatalysts with heteroatomic coordination structures by using two or more heteroatoms coordinated to the active center metal atom. It was found that this asym-metric coordination structure effectively modulated the electronic structure of the central metal atom,optimizing the adsorption and desorption energies of the catalytic reaction,and improving the electrocatalytic performance. This paper presents a comprehensive review of the synthesis strategies and characterization techniques of carbon-based single-atom electrocatalysts with heteroatomic coordination structures,and their structure-property correlation for energy electrocatalysis. We give prospects of the future research for this field at the end of the review.
WOS关键词FE-N-C ; OXYGEN REDUCTION REACTION ; ELECTROCHEMICAL CO2 REDUCTION ; METAL-ORGANIC FRAMEWORK ; ACTIVE-SITES ; EFFICIENT ELECTROREDUCTION ; ELECTRONIC-STRUCTURE ; NITROGEN REDUCTION ; HYDROGEN EVOLUTION ; RATIONAL DESIGN
资助项目National Natural Science Foundation of China[51932001] ; National Natural Science Foundation of China[51872024] ; National Natural Science Foundation of China[52022097] ; National Key Research and Development Program of China[2018YFA0703503] ; Foundation of the Youth Innovation Promotion Association of Chinese Academy of Sciences[2020048]
WOS研究方向Chemistry
语种英语
出版者HIGHER EDUCATION PRESS
WOS记录号WOS:000819185600001
资助机构National Natural Science Foundation of China ; National Key Research and Development Program of China ; Foundation of the Youth Innovation Promotion Association of Chinese Academy of Sciences
源URL[http://ir.ipe.ac.cn/handle/122111/54094]  
专题中国科学院过程工程研究所
通讯作者WAN Jiawei; YU Ranbo
作者单位1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
2.Univ Sci & Technol Beijing, Sch Met & Ecol Engn, Beijing 100083, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714		 XIA Tian,WAN Jiawei,YU Ranbo. Progress of the Structure-property Correlation of Heteroatomic Coordination Structured Carbon-based Single-atom Electrocatalysts[J]. CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,2022,43(5):21.
APA XIA Tian,WAN Jiawei,&YU Ranbo.(2022).Progress of the Structure-property Correlation of Heteroatomic Coordination Structured Carbon-based Single-atom Electrocatalysts.CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,43(5),21.
MLA XIA Tian,et al."Progress of the Structure-property Correlation of Heteroatomic Coordination Structured Carbon-based Single-atom Electrocatalysts".CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE 43.5(2022):21.

入库方式： OAI收割

来源：过程工程研究所

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