Photothermal catalytic oxidation of toluene with enhanced efficiency over constructed CuMn2O4/Mn2O3 heterojunction catalyst
文献类型:期刊论文
作者 | Nie, Linfeng1; Li, Shuangde1; Chai, Shaohua1,2; Han, Ning; Chen, Yunfa1,2 |
刊名 | APPLIED SURFACE SCIENCE |
出版日期 | 2022-12-15 |
卷号 | 605页码:9 |
ISSN号 | 0169-4332 |
关键词 | Photothermal catalyst VOC Heterojunction |
DOI | 10.1016/j.apsusc.2022.154567 |
英文摘要 | Photothermal catalyst oxidation of VOCs is a hot issue in the air purifier field due to the reducing of secondary energy consumption. Herein, we reported a photothermal catalyst CuMn2O4/Mn2O3 with heterojunction for catalytic oxidizing toluene with high efficiency through sol-gel method followed different calcination temperature. Under the irradiation of 700 mW/cm(2) Xe lamp simulated sun light, the CuMn2O4/Mn2O3 catalyst exhibited excellent full spectrum light absorption capacity, photo-thermal conversion ability and toluene conversion performance with a 90% toluene conversion (T = 233 degrees C, WHSV = 30,000 mL/gmiddoth), together with a good catalytic stability. The excellent performance can be attributed to the synergistic effect of abundant oxygen vacancies, Mn3+ active sites and heterojunctions between CuMn2O4 and Mn2O3 due to the XPS, H-2-TPR, UPS characterizations. |
WOS关键词 | CORE-SHELL ; TEMPERATURE ; REMOVAL ; OXIDES ; CU ; CARBON ; GAS ; VOC |
资助项目 | Fund of State Key Laboratory of Multi -phase Complex Systems[MPCS-2021-A- 01] ; Strategic Priority Research Program (A) of the Chinese Academy of Sciences[XDA23030300] ; Cultivating Project of Strategic Priority Research Program of Chinese Academy of Sciences[XDPB19] ; Youth Innovation Promotion Association of Chinese Academy of Sciences |
WOS研究方向 | Chemistry ; Materials Science ; Physics |
语种 | 英语 |
出版者 | ELSEVIER |
WOS记录号 | WOS:000860475400006 |
资助机构 | Fund of State Key Laboratory of Multi -phase Complex Systems ; Strategic Priority Research Program (A) of the Chinese Academy of Sciences ; Cultivating Project of Strategic Priority Research Program of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences |
源URL | [http://ir.ipe.ac.cn/handle/122111/54777] |
专题 | 中国科学院过程工程研究所 |
通讯作者 | Li, Shuangde; Chen, Yunfa |
作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Coll Mat Sci & Optoelect Technol, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Nie, Linfeng,Li, Shuangde,Chai, Shaohua,et al. Photothermal catalytic oxidation of toluene with enhanced efficiency over constructed CuMn2O4/Mn2O3 heterojunction catalyst[J]. APPLIED SURFACE SCIENCE,2022,605:9. |
APA | Nie, Linfeng,Li, Shuangde,Chai, Shaohua,Han, Ning,&Chen, Yunfa.(2022).Photothermal catalytic oxidation of toluene with enhanced efficiency over constructed CuMn2O4/Mn2O3 heterojunction catalyst.APPLIED SURFACE SCIENCE,605,9. |
MLA | Nie, Linfeng,et al."Photothermal catalytic oxidation of toluene with enhanced efficiency over constructed CuMn2O4/Mn2O3 heterojunction catalyst".APPLIED SURFACE SCIENCE 605(2022):9. |
入库方式: OAI收割
来源:过程工程研究所
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