Ultralow Friction and High Robustness of Monolayer Ionic Liquids
文献类型：期刊论文
| 作者 | Lu, Yumiao2,3; Wang, Yanlei2,3; Huo, Feng2,3; Chen, Wei2; Ma, Ming1; Ding, Wei-Lu2,3; He, Hongyan2,3,4; Zhang, Suojiang2,3,4 |
| 刊名 | ACS NANO
 |
| 出版日期 | 2022-10-12 |
| 页码 | 10 |
| 关键词 | monolayer ionic liquid self-assembly ordered structure ultralow friction robustness |
| ISSN号 | 1936-0851 |
| DOI | 10.1021/acsnano.2c05779 |
| 英文摘要 | Ultralow friction between interacting surfaces in relative motion is of vital importance in many pure and applied sciences. We found that surfaces bearing ordered monolayer ionic liquids (ILs) can have friction coefficient mu values as low as 0.001 at pressures up to 78 MPa and exhibit good structure recoverability. This extreme lubrication is attributed primarily to the ordered striped structure driven by the "atomic-locking" effect between carbon atoms on the alkyl chain of ILs and graphite. The longer alkyl chain has lower mu values, and the stripe periodicity is decisive in reducing energy dissipation during the sliding process. In combination with simulation, the alternate atomic-scale ordered and disordered ionic regions were recognized, whose ratio fundamentally determines the mu values and lubrication mechanism. This finding is an important step toward the practical utilization of ILs with negligible vapor pressure as superlubricating materials in future technological applications operating under extreme conditions. |
| WOS关键词 | MOLECULAR-DYNAMICS ; MICELLE FORMATION ; LUBRICATION ; FORCE ; FILMS ; ORGANIZATION ; AGGREGATION ; SIMULATION ; SURFACES |
| 资助项目 | National Key Research and Development Program of China[2021YFB3802600] ; National Natural Science Foundation of China[21922813] ; National Natural Science Foundation of China[21908221] ; National Natural Science Foundation of China[21890762] ; Fund of State Key Laboratory of Multiphase complex systems[MPCS-2021-A-07] ; Youth Innovation Promotion Association CAS[2021046] ; Youth Innovation Promotion Association CAS[Y2021022] |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science |
| 语种 | 英语 |
| WOS记录号 | WOS:000870268800001 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | National Key Research and Development Program of China ; National Natural Science Foundation of China ; Fund of State Key Laboratory of Multiphase complex systems ; Youth Innovation Promotion Association CAS |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/55129]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Ma, Ming; He, Hongyan; Zhang, Suojiang |
| 作者单位 | 1.Tsinghua Univ, Ctr Nano & Micro Mech, Dept Mech Engn, State Key Lab Tribol Adv Equipment SKLT, Beijing 100084, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst,CAS Key Lab, Beijing 100190, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 4.Chinese Acad Sci, Innovat Acad Green Manufacture, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lu, Yumiao,Wang, Yanlei,Huo, Feng,et al. Ultralow Friction and High Robustness of Monolayer Ionic Liquids[J]. ACS NANO,2022:10. |
| APA | Lu, Yumiao.,Wang, Yanlei.,Huo, Feng.,Chen, Wei.,Ma, Ming.,...&Zhang, Suojiang.(2022).Ultralow Friction and High Robustness of Monolayer Ionic Liquids.ACS NANO,10. |
| MLA | Lu, Yumiao,et al."Ultralow Friction and High Robustness of Monolayer Ionic Liquids".ACS NANO (2022):10. |
入库方式： OAI收割
来源：过程工程研究所
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