Fabrication of CdxZn1-xS@VPO (x=0.2) Nanocomposites for n-Butane Selective Oxidation Toward Maleic Anhydride
文献类型:期刊论文
作者 | Faizan, Muhammad1,2; Saeed, Aamir1,2; Song, Piao1,2; Zhang, Ruirui2; Liu, Ruixia1,2,3; Chang, Zhi4; Wu, Liuzhu4; Zhang, Manyuan4 |
刊名 | CATALYSIS LETTERS
![]() |
出版日期 | 2022-11-05 |
页码 | 18 |
关键词 | Cd0.2Zn0.8S@VPO nanocomposites Vanadium phosphorus oxide n-Butane selective oxidation Structure directing agent Electronic promoting agent |
ISSN号 | 1011-372X |
DOI | 10.1007/s10562-022-04170-5 |
英文摘要 | Vanadium phosphorous oxide (VPO) catalysts have been recognized as heterogeneous catalyst for selective oxidation of lowcarbon alkanes i.e., n-butane toward maleic anhydride. This process has widely gained attention globally due to its highly selective and cost-effective process. Herein, we employed Cd0.2Zn0.8S as a support for the VPO catalyst and evaluated its n-butane catalytic performance. Compared to the unpromoted catalyst (Blank-VPO), a higher n-butane conversion and MA yield were successfully obtained from the promoted catalyst (Cd0.2Zn0.8S@VPO). Interestingly, it reduces the byproducts, i.e., CO2 and CO emission. Characterization methods such as TGA, XRD, EDS, SEM, FTIR, NH3-TPD, XPS, TEM, and Raman spectroscopy were used to characterize the Cd0.2Zn0.8S, VPO precursor and catalyst. [GRAPHICS] . |
WOS关键词 | PHOSPHORUS OXIDE CATALYST ; VANADIUM PHOSPHATE ; MILD OXIDATION ; VPO CATALYSTS ; PERFORMANCE ; PYROPHOSPHATE ; ACTIVATION ; SOLVENTS ; PHASE ; MO |
资助项目 | Key Scientific and Technological Projects in Huizhou[2021JBZ5.1] ; Yulin University[2021016] ; Dalian National Laboratory for Clean Energy[2021016] ; Innovation Academy for Green Manufacture of Chinese Academy of Science[IAGM2020C17] |
WOS研究方向 | Chemistry |
语种 | 英语 |
WOS记录号 | WOS:000878923000001 |
出版者 | SPRINGER |
资助机构 | Key Scientific and Technological Projects in Huizhou ; Yulin University ; Dalian National Laboratory for Clean Energy ; Innovation Academy for Green Manufacture of Chinese Academy of Science |
源URL | [http://ir.ipe.ac.cn/handle/122111/55513] ![]() |
专题 | 中国科学院过程工程研究所 |
通讯作者 | Faizan, Muhammad; Liu, Ruixia |
作者单位 | 1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, CAS Key Lab Green Proc & Engn, State Key Lab Multiphase Complex Syst,Inst Proc E, Beijing 100190, Peoples R China 3.Zhengzhou Inst Emerging Ind Technol, Zhengzhou 450000, Peoples R China 4.Pangang Grp Vanadium & Titanium Resources Co Ltd, Panzhihua 617000, Peoples R China |
推荐引用方式 GB/T 7714 | Faizan, Muhammad,Saeed, Aamir,Song, Piao,et al. Fabrication of CdxZn1-xS@VPO (x=0.2) Nanocomposites for n-Butane Selective Oxidation Toward Maleic Anhydride[J]. CATALYSIS LETTERS,2022:18. |
APA | Faizan, Muhammad.,Saeed, Aamir.,Song, Piao.,Zhang, Ruirui.,Liu, Ruixia.,...&Zhang, Manyuan.(2022).Fabrication of CdxZn1-xS@VPO (x=0.2) Nanocomposites for n-Butane Selective Oxidation Toward Maleic Anhydride.CATALYSIS LETTERS,18. |
MLA | Faizan, Muhammad,et al."Fabrication of CdxZn1-xS@VPO (x=0.2) Nanocomposites for n-Butane Selective Oxidation Toward Maleic Anhydride".CATALYSIS LETTERS (2022):18. |
入库方式: OAI收割
来源:过程工程研究所
浏览0
下载0
收藏0
其他版本
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。