中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Simultaneous Fe(OH)(3) formation and silicon adsorption removal from reverse osmosis brine wastewater

文献类型:期刊论文

作者Sun, Jingjing1,2; Chen, Shangqing1; Wang, Junfeng1,3; Nie, Yi1,3
刊名CHEMICAL ENGINEERING RESEARCH & DESIGN
出版日期2022-12-01
卷号188页码:964-971
关键词Silicon removal Reverse osmosis brine Fe(OH)3 Adsorption
ISSN号0263-8762
DOI10.1016/j.cherd.2022.10.0420263-8762
英文摘要The reduce of the silicon concentration to low level (< 5 mg center dot L-1) from the reverse osmosis brine wastewater is challenging and desirable for the maintain the membrane life and performance, as well as the wastewater treatment costs. This work focuses on the removal of silicon from the reverse osmosis brine wastewater by adding FeCl3 into the plant wastewater for simultaneous Fe(OH)3 formation and silicon adsorption. The effects of pH, FeCl3 dosing concentration, reaction time, and temperature on the silicon removal ratio were investigated. It was demonstrated that the silicon removal ratio could reach up to 94% and its residual concentration was 3.2 mg center dot L-1, which met the require of water quality in the reverse osmosis system. These results showed that Fe(OH)3 could effectively be formed by adding FeCl3 and realize the efficient silicon removal from the reverse osmosis brine wastewater, even when chloride ion (Cl-), sulfate anion (SO42-) and nitrate ion (NO3-) were present. Moreover, the adsorption thermodynamics, kinetics and isotherms during the process of the adsorption of silicon from the wastewater by Fe(OH)3 were studied. The calculated adsorption capacity of silicon could reach 612.74 mg center dot g-1, which was much larger than those of reported adsorbents. These results showed that the silicon removal process was spontaneously exothermic and mainly controlled by the physical adsorption and the monomolecular layer adsorption. This simple and cost-effective method could be used for the silicon removal from different kinds of Si-containing wastewater. (c) 2022 Institution of Chemical Engineers. Published by Elsevier Ltd. All rights reserved.
WOS关键词BRACKISH-WATER ; SCALE MITIGATION ; DESALINATION ; PRETREATMENT ; RECOVERY ; PRECIPITATION ; ELECTROCOAGULATION ; PERFORMANCE ; BEHAVIOR ; ACID
资助项目National Key R & D Program of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; [2021YFC3201404] ; [21978302] ; [U20A20149] ; [2021TQ0333] ; [2022M713174]
WOS研究方向Engineering
语种英语
WOS记录号WOS:000893764400003
出版者ELSEVIER
资助机构National Key R & D Program of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation
源URL[http://ir.ipe.ac.cn/handle/122111/56038]  
专题中国科学院过程工程研究所
通讯作者Wang, Junfeng; Nie, Yi
作者单位1.Chinese Acad Sci, Inst Proc Engn, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
2.Shenyang Univ Chem Technol, Sch Chem Engn, Shenyang 110142, Liaoning, Peoples R China
3.Chinese Acad Sci, Innovat Acad Green Manufacture, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Sun, Jingjing,Chen, Shangqing,Wang, Junfeng,et al. Simultaneous Fe(OH)(3) formation and silicon adsorption removal from reverse osmosis brine wastewater[J]. CHEMICAL ENGINEERING RESEARCH & DESIGN,2022,188:964-971.
APA Sun, Jingjing,Chen, Shangqing,Wang, Junfeng,&Nie, Yi.(2022).Simultaneous Fe(OH)(3) formation and silicon adsorption removal from reverse osmosis brine wastewater.CHEMICAL ENGINEERING RESEARCH & DESIGN,188,964-971.
MLA Sun, Jingjing,et al."Simultaneous Fe(OH)(3) formation and silicon adsorption removal from reverse osmosis brine wastewater".CHEMICAL ENGINEERING RESEARCH & DESIGN 188(2022):964-971.

入库方式: OAI收割

来源:过程工程研究所

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