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Pollution characteristics and health risk assessment of polycyclic aromatic hydrocarbons and nitrated polycyclic aromatic hydrocarbons during heating season in Beijing

文献类型：期刊论文

作者Bai, Xurong2,3; Wei, Jie1; Ren, Yanqin2; Gao, Rui2; Chai, Fahe2; Li, Hong2; Xu, Fei3; Kong, Yuxue2
刊名JOURNAL OF ENVIRONMENTAL SCIENCES
出版日期2023
卷号123页码:169-182
ISSN号1001-0742
关键词Heating season Polycyclic aromatic hydrocarbons Nitrated polycyclic aromatic hydrocarbons Pollution characteristics Source Health risk assessment
DOI10.1016/j.jes.2022.02.047
通讯作者Ren, Yanqin(renyq@craes.org.cn) ; Gao, Rui(gaorui@craes.org.cn)
英文摘要Polycyclic aromatic hydrocarbons (PAHs) and their nitrated derivatives (NPAHs) attract continuous attention due to their outstanding carcinogenicity and mutagenicity. In order to investigate the diurnal variations, sources, formation mechanism, and health risk assessment of them in heating season, particulate matter (PM) were collected in Beijing urban area from December 26, 2017 to January 17, 2018. PAHs and NPAHs in PM were quantitatively analyzed via gas chromatography-mass spectrometry (GC-MS). Average daily concentrations of PAHs and NPAHs were (78 +/- 54) ng/m(3) and (783 +/- 684) pg/m(3), respectively. The concentrations of them were significantly higher at nighttime than at daytime, and NPAHs concentrations were 1-2 orders of magnitude lower than PAHs concentrations. In the heating season, the dominant species of PAHs include benzo[b]fluoranthene, fluoranthene, pyrene, and chrysene, while 9-nitroanthracene, 2+3-nitrofluoranthene, and 2-nitropyrene were dominant species for NPAHs. NPAHs were found to have a single peak during heating and to be primarily distributed in the 0.4-0.7 mu m particle size. Primary emissions such as biomass burning, coal combustion, and traffic emissions were the major sources of PAHs. NPAHs were produced by the primary source of vehicle emissions and the secondary reaction triggered by OH radicals, as well as biomass burning during daytime. According to the health risk assessment, the total carcinogenic risk was higher in adults than in children. While upon oral ingestion, the carcinogenic risk in children was higher than that of adults, but the risk of adults was higher than children through skin contact and respiratory inhalation. (c) 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
WOS关键词AIRBORNE PARTICULATE MATTER ; AMBIENT AIR ; PM2.5-BOUND PAHS ; OXYGENATED-PAHS ; SUBURBAN SITES ; BOUND PAHS ; SIZE DISTRIBUTION ; NITRO-PAHS ; URBAN ; CHINA
资助项目National Natural Science Foundation of China[41907197] ; Fundamental Research Funds for Central Public Welfare Scientific Research Institutes of China, Chinese Research Academy of Environmental Sciences[2019YSKY-018] ; National Key R&D Program of China[2019YFC0214800] ; Standard System and Key Standards Research of National Ecological Environment Protection and Risk Prevention[2020YFC18063]
WOS研究方向Environmental Sciences & Ecology
语种英语
出版者SCIENCE PRESS
WOS记录号WOS:000911675700014
资助机构National Natural Science Foundation of China ; Fundamental Research Funds for Central Public Welfare Scientific Research Institutes of China, Chinese Research Academy of Environmental Sciences ; National Key R&D Program of China ; Standard System and Key Standards Research of National Ecological Environment Protection and Risk Prevention
源URL[http://ir.igsnrr.ac.cn/handle/311030/189760]  
专题中国科学院地理科学与资源研究所
通讯作者Ren, Yanqin; Gao, Rui
作者单位1.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Key Lab Ecosyst Network Observat & Modeling, Beijing 100101, Peoples R China
2.Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China
3.Shandong Univ, Environm Res Inst, Qingdao 266237, Peoples R China
推荐引用方式
GB/T 7714		 Bai, Xurong,Wei, Jie,Ren, Yanqin,et al. Pollution characteristics and health risk assessment of polycyclic aromatic hydrocarbons and nitrated polycyclic aromatic hydrocarbons during heating season in Beijing[J]. JOURNAL OF ENVIRONMENTAL SCIENCES,2023,123:169-182.
APA Bai, Xurong.,Wei, Jie.,Ren, Yanqin.,Gao, Rui.,Chai, Fahe.,...&Kong, Yuxue.(2023).Pollution characteristics and health risk assessment of polycyclic aromatic hydrocarbons and nitrated polycyclic aromatic hydrocarbons during heating season in Beijing.JOURNAL OF ENVIRONMENTAL SCIENCES,123,169-182.
MLA Bai, Xurong,et al."Pollution characteristics and health risk assessment of polycyclic aromatic hydrocarbons and nitrated polycyclic aromatic hydrocarbons during heating season in Beijing".JOURNAL OF ENVIRONMENTAL SCIENCES 123(2023):169-182.

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来源：地理科学与资源研究所

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