Chlortetracycline hydrochloride removal by different biochar/Fe composites: A comparative study
文献类型：期刊论文
| 作者 | Zhao, Nan; Liu, Kunyuan; Yan, Bofang; Zhu, Ling; Zhao, Chuanfang; Gao, Jia; Ruan, Jujun; Zhang, Weihua; Qiu, Rongliang |
| 刊名 | JOURNAL OF HAZARDOUS MATERIALS
 |
| 出版日期 | 2021-02-05 |
| 卷号 | 403页码:- |
| 关键词 | Biochar/Fe composites Chlortetracycline hydrochloride Adsorption and degradation Cost analysis Principal component analysis Comprehensive assessment |
| ISSN号 | 0304-3894 |
| 英文摘要 | In the last years, the synthesis and applications of biochar/Fe composites have been extensively studied, but only few papers have systematically evaluated their removal performances. Herein, we successfully synthesized and structurally characterized Fe-0, Fe3C, and Fe3O4-coated biochars (BCs) for the removal of chlortetracycline hydrochloride (CH). Evaluation of their removal rate and affinity revealed that Fe-0@BC could achieve better and faster CH removal and degradation than Fe3C@BC and Fe3O4@BC. The removal rate was controlled by the O-Fe content and solution pH after the reaction. The CH adsorption occurred on the O-C groups of Fe-0@BC and the O=C and O-Fe groups of Fe3C@BC and Fe3O4@BC. Electron paramagnetic resonance analysis and radical quenching experiments indicated that HO center dot and O-1(2)/O-2(center dot-) were mainly responsible for CH degradation by biochar/Fe composites. Additional parameters, such as effects of initial concentrations and coexisting anions, regeneration capacity, cost and actual wastewater treatment were also explored. Principal component analysis was applied for a comprehensive and quantitative assessment of the three materials, indicating Fe-0@BC is the most beneficial functional material for CH removal. |
| WOS研究方向 | Engineering, Environmental ; Environmental Sciences |
| 源URL | [http://ir.rcees.ac.cn/handle/311016/45686]  |
| 专题 | 生态环境研究中心_环境化学与生态毒理学国家重点实验室 |
| 作者单位 | 1.Tongji Univ, Coll Environm Sci & Engn, State Key Lab Pollut Control & Resource Reuse, Shanghai 200092, Peoples R China 2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China 3.South China Agr Univ, Coll Nat Resources & Environm, Guangdong Lab Lingnan Modern Agr, Guangzhou 510642, Peoples R China 4.Sun Yat Sen Univ, Guangdong Prov Key Lab Environm Pollut Control &, Sch Environm Sci & Engn, Guangzhou 510275, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Nan,Liu, Kunyuan,Yan, Bofang,et al. Chlortetracycline hydrochloride removal by different biochar/Fe composites: A comparative study[J]. JOURNAL OF HAZARDOUS MATERIALS,2021,403:-. |
| APA | Zhao, Nan.,Liu, Kunyuan.,Yan, Bofang.,Zhu, Ling.,Zhao, Chuanfang.,...&Qiu, Rongliang.(2021).Chlortetracycline hydrochloride removal by different biochar/Fe composites: A comparative study.JOURNAL OF HAZARDOUS MATERIALS,403,-. |
| MLA | Zhao, Nan,et al."Chlortetracycline hydrochloride removal by different biochar/Fe composites: A comparative study".JOURNAL OF HAZARDOUS MATERIALS 403(2021):-. |
入库方式： OAI收割
来源：生态环境研究中心
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