中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Efficient removal of bisphenol S by non-radical activation of peroxydisulfate in the presence of nano-graphite

文献类型:期刊论文

作者Zhang, Ziyu; Huang, Xiaoyan; Ma, Jie; Pei, Zhiguo; Luo, Lei; Ke, Xin; Qin, Fei; Li, Yingming; Yang, Ruiqiang; Zhu, Ying
刊名WATER RESEARCH
出版日期2021-08-01
卷号201页码:-
关键词Nano-graphite Peroxydisulfate Bisphenol S Non-radical pathway Degradation
ISSN号0043-1354
英文摘要An environmentally friendly and efficient catalyst is important for the persulfate activation and pollutants removal from water. In this study, nano-graphite (NG) prepared by detonation method, was firstly applied as the superb carbon catalyst to activate peroxydisulfate (PDS) for the degradation of bisphenol S (BPS) via a nonradical pathway. Results showed that NG had a very high catalytic performance and degraded most of BPS within 20.0 min, out-performing many popular metal-based catalysts. The doped N atoms (i.e. graphitic N and pyridinic N) in NG were identified as the possible reactive sites for the PDS activation. It is proposed that PDS could form the metastable surface-bound PDS complexes on the NG surface, which promoted the BPS degradation. The NG/PDS system had a strong anti-interference ability for the environmental background substances and a wide operative pH range, so it had a good application prospect in the actual wastewater environment. This study not only provides an efficient method for the removal of bisphenol pollutants, but also deepens the insight into the reaction mechanisms.
WOS研究方向Engineering, Environmental ; Environmental Sciences ; Water Resources
源URL[http://ir.rcees.ac.cn/handle/311016/45717]  
专题生态环境研究中心_环境化学与生态毒理学国家重点实验室
作者单位1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, POB 2871, Beijing 100085, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Shenyang Aerosp Univ, Coll Energy & Environm, Shenyang 110136, Peoples R China
4.Beijing Union Univ, Coll Biochem Engn, Beijing 100023, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Ziyu,Huang, Xiaoyan,Ma, Jie,et al. Efficient removal of bisphenol S by non-radical activation of peroxydisulfate in the presence of nano-graphite[J]. WATER RESEARCH,2021,201:-.
APA Zhang, Ziyu.,Huang, Xiaoyan.,Ma, Jie.,Pei, Zhiguo.,Luo, Lei.,...&Zhang, Qinghua.(2021).Efficient removal of bisphenol S by non-radical activation of peroxydisulfate in the presence of nano-graphite.WATER RESEARCH,201,-.
MLA Zhang, Ziyu,et al."Efficient removal of bisphenol S by non-radical activation of peroxydisulfate in the presence of nano-graphite".WATER RESEARCH 201(2021):-.

入库方式: OAI收割

来源:生态环境研究中心

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