Efficient removal of bisphenol S by non-radical activation of peroxydisulfate in the presence of nano-graphite
文献类型:期刊论文
作者 | Zhang, Ziyu; Huang, Xiaoyan; Ma, Jie; Pei, Zhiguo![]() |
刊名 | WATER RESEARCH
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出版日期 | 2021-08-01 |
卷号 | 201页码:- |
关键词 | Nano-graphite Peroxydisulfate Bisphenol S Non-radical pathway Degradation |
ISSN号 | 0043-1354 |
英文摘要 | An environmentally friendly and efficient catalyst is important for the persulfate activation and pollutants removal from water. In this study, nano-graphite (NG) prepared by detonation method, was firstly applied as the superb carbon catalyst to activate peroxydisulfate (PDS) for the degradation of bisphenol S (BPS) via a nonradical pathway. Results showed that NG had a very high catalytic performance and degraded most of BPS within 20.0 min, out-performing many popular metal-based catalysts. The doped N atoms (i.e. graphitic N and pyridinic N) in NG were identified as the possible reactive sites for the PDS activation. It is proposed that PDS could form the metastable surface-bound PDS complexes on the NG surface, which promoted the BPS degradation. The NG/PDS system had a strong anti-interference ability for the environmental background substances and a wide operative pH range, so it had a good application prospect in the actual wastewater environment. This study not only provides an efficient method for the removal of bisphenol pollutants, but also deepens the insight into the reaction mechanisms. |
WOS研究方向 | Engineering, Environmental ; Environmental Sciences ; Water Resources |
源URL | [http://ir.rcees.ac.cn/handle/311016/45717] ![]() |
专题 | 生态环境研究中心_环境化学与生态毒理学国家重点实验室 |
作者单位 | 1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, POB 2871, Beijing 100085, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Shenyang Aerosp Univ, Coll Energy & Environm, Shenyang 110136, Peoples R China 4.Beijing Union Univ, Coll Biochem Engn, Beijing 100023, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Ziyu,Huang, Xiaoyan,Ma, Jie,et al. Efficient removal of bisphenol S by non-radical activation of peroxydisulfate in the presence of nano-graphite[J]. WATER RESEARCH,2021,201:-. |
APA | Zhang, Ziyu.,Huang, Xiaoyan.,Ma, Jie.,Pei, Zhiguo.,Luo, Lei.,...&Zhang, Qinghua.(2021).Efficient removal of bisphenol S by non-radical activation of peroxydisulfate in the presence of nano-graphite.WATER RESEARCH,201,-. |
MLA | Zhang, Ziyu,et al."Efficient removal of bisphenol S by non-radical activation of peroxydisulfate in the presence of nano-graphite".WATER RESEARCH 201(2021):-. |
入库方式: OAI收割
来源:生态环境研究中心
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