中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Migration mechanism and risk assessment of chlorinated paraffins in highly polluted Ya'Er lake area, China

文献类型:期刊论文

作者Li, Chang; Chen, Lufeng; He, Yujian; Liang, Yong; Wang, Yingjun; Li, Feifei; Gao, Wei; Wang, Yawei; Jiang, Guibin
刊名ENVIRONMENTAL POLLUTION
出版日期2021-07-15
卷号281页码:-
ISSN号0269-7491
关键词Highly polluted areas Chlorinated paraffins Distribution Migration mechanism Risk assessment
英文摘要Chlorinated paraffins (CPs), a type of toxic and persistent organic substances, can persist in environmental media for a long time and have adverse effects on human health. Thus, it is of great importance to investigate the accumulation and environmental behavior of CPs in industrial areas. In this study, farmland soil, water, and sediment core samples from abandoned oxidation ponds used by three chemical plants to treat wastewater over the past 38 years were investigated in detail. Results show that the concentration of CPs in sediments varied significantly with the water flow direction. The oxidation pond closest to a sewage outlet had the highest concentrations of short-chain chlorinated paraffin (SCCPs) and medium-chain chlorinated paraffin (MCCPs), within the ranges of 44.0-6.21 x 10(4) ng/g dw (mean 9.32 x 10(3) ng/g dw) and 143-1.30 x 10(6) ng/g dw (mean 1.22 x 10(5) ng/g dw), respectively. However, in the oxidation pond farthest from the sewage outlet, CP concentrations in sediments were significantly reduced, with Sigma SCCPs and Sigma MCCPs concentrations ranging from N.D.-249 ng/g dw (mean 66.8 ng/g dw) and N.D.-222 ng/g dw (mean 34.0 ng/g dw), respectively. Moreover, MCCP level in the water was below the detection limit, while the concentration of SCCP ranged from 41.0 to 1.53 x 10(3) ng/L (mean 267 ng/L). Finally, a remarkable spatial trend and specific congener distribution were observed in the sediment test results. The horizontal and vertical distributions of the sediments indicate that short-chain (C-10-(11)) and low-chlorinated (Cl-6-(7)) homologs are more likely to migrate deeper or farther away from the pollution source. (C) 2021 Elsevier Ltd. All rights reserved.
WOS研究方向Environmental Sciences
源URL[http://ir.rcees.ac.cn/handle/311016/45783]  
专题生态环境研究中心_环境化学与生态毒理学国家重点实验室
作者单位1.Jianghan Univ, Inst Environm & Hlth, Hubei Key Lab Environm & Hlth Effects Persistent, Wuhan 430056, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China
4.UCAS, Hangzhou Inst Adv Study, Sch Environm, Hangzhou 310000, Peoples R China
推荐引用方式
GB/T 7714
Li, Chang,Chen, Lufeng,He, Yujian,et al. Migration mechanism and risk assessment of chlorinated paraffins in highly polluted Ya'Er lake area, China[J]. ENVIRONMENTAL POLLUTION,2021,281:-.
APA Li, Chang.,Chen, Lufeng.,He, Yujian.,Liang, Yong.,Wang, Yingjun.,...&Jiang, Guibin.(2021).Migration mechanism and risk assessment of chlorinated paraffins in highly polluted Ya'Er lake area, China.ENVIRONMENTAL POLLUTION,281,-.
MLA Li, Chang,et al."Migration mechanism and risk assessment of chlorinated paraffins in highly polluted Ya'Er lake area, China".ENVIRONMENTAL POLLUTION 281(2021):-.

入库方式: OAI收割

来源:生态环境研究中心

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