Unexpected Persistent Production of Reactive Oxygen Species during the Degradation of Black Phosphorous in the Darkness
文献类型:期刊论文
作者 | Yu, Wanchao; Xu, Jin![]() ![]() ![]() ![]() |
刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
![]() |
出版日期 | 2022 |
卷号 | 61期号:47页码:1-5 |
关键词 | Chemiluminescence Dark Conditions Few-Layer Black Phosphorus Reactive Oxygen Species Self-Degradation |
ISSN号 | 1433-7851 |
英文摘要 | Few-layer black phosphorus (FLBP) is easily degraded under ambient conditions which is problem that hinders the application of FLBP, but its degradation mechanism is not yet well understood. In this work, we surprisingly found that persistent generation of reactive oxygen species (ROS) was involved in FLBP degradation even in the dark. The ROS generation patterns and mechanism were revealed by chemiluminescence (CL) and density functional theory (DFT). Meanwhile, rhodamine B (RhB) and methyl orange (MO) can also be removed by FLBP under dark conditions, which further shows the ROS generation during FLBP self-degradation. This work provides new insights into the FLBP self-degradation mechanism and opens opportunities to practically implement FLBP for green catalytic application. |
源URL | [https://ir.rcees.ac.cn/handle/311016/48523] ![]() |
专题 | 生态环境研究中心_环境化学与生态毒理学国家重点实验室 |
作者单位 | 1.University of Chinese Academy of Sciences, CAS 2.Chinese Academy of Sciences 3.Research Center for Eco-Environmental Sciences (RCEES) 4.Jianghan University |
推荐引用方式 GB/T 7714 | Yu, Wanchao,Xu, Jin,Chen, Fengjie,et al. Unexpected Persistent Production of Reactive Oxygen Species during the Degradation of Black Phosphorous in the Darkness[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2022,61(47):1-5. |
APA | Yu, Wanchao.,Xu, Jin.,Chen, Fengjie.,Wang, Yarui.,Tang, Shanshan.,...&Wang, Yawei.(2022).Unexpected Persistent Production of Reactive Oxygen Species during the Degradation of Black Phosphorous in the Darkness.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,61(47),1-5. |
MLA | Yu, Wanchao,et al."Unexpected Persistent Production of Reactive Oxygen Species during the Degradation of Black Phosphorous in the Darkness".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 61.47(2022):1-5. |
入库方式: OAI收割
来源:生态环境研究中心
浏览0
下载0
收藏0
其他版本
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。