Constructing and selecting optimal sustainable sanitation system based on expanded structured decision-making for global sanitation and resources crisis
文献类型:期刊论文
作者 | Hu, Ming; Xiao, Jinyu; Fan, Bin; Sun, Wei; Zhu, Shikun |
刊名 | JOURNAL OF CLEANER PRODUCTION
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出版日期 | 2021-12-10 |
卷号 | 21期号:20页码:15809-15826 |
ISSN号 | 1680-7316 |
英文摘要 | We compare Community Multiscale Air Quality (CMAQ) model predictions with measured nitrous acid (HONO) concentrations in Beijing, China, for December 2015. The model with the existing HONO chemistry in CMAQ severely underestimates the observed HONO concentrations with a normalized mean bias of 97 %. We revise the HONO chemistry in the model by implementing six additional heterogeneous reactions in the model: the reaction of nitrogen dioxide (NO2) on ground surfaces, the reaction of NO2 on aerosol surfaces, the reaction of NO2 on soot surfaces, the photolysis of aerosol nitrate, the nitric acid displacement reaction, and the hydrochloric acid displacement reaction. The model with the revised chemistry substantially increases HONO predictions and improves the comparison with observed data with a normalized mean bias of 5 %. The photolysis of HONO enhances daytime hydroxyl radical by almost a factor of 2. The enhanced hydroxyl radical concentrations compare favorably with observed data and produce additional sulfate via the reaction with sulfur dioxide, aerosol nitrate via the reaction with nitrogen dioxide, and ganic compounds. The additional sulfate stemming from revised HONO chemistry improves the comparison with observed concentration; however, it does not close the gap between model prediction and the observation during polluted days. |
源URL | [https://ir.rcees.ac.cn/handle/311016/46844] ![]() |
专题 | 生态环境研究中心_环境水质学国家重点实验室 |
作者单位 | 1.Univ Regina, Fac Engn & Appl Sci, Environm Syst Engn Program, Regina, SK S4S 0A2, Canada 2.Water Sci & Technol Res Inst Beijing, Beijing 100048, Peoples R China 3.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Aquat Chem, Beijing 100085, Peoples R China 4.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China |
推荐引用方式 GB/T 7714 | Hu, Ming,Xiao, Jinyu,Fan, Bin,et al. Constructing and selecting optimal sustainable sanitation system based on expanded structured decision-making for global sanitation and resources crisis[J]. JOURNAL OF CLEANER PRODUCTION,2021,21(20):15809-15826. |
APA | Hu, Ming,Xiao, Jinyu,Fan, Bin,Sun, Wei,&Zhu, Shikun.(2021).Constructing and selecting optimal sustainable sanitation system based on expanded structured decision-making for global sanitation and resources crisis.JOURNAL OF CLEANER PRODUCTION,21(20),15809-15826. |
MLA | Hu, Ming,et al."Constructing and selecting optimal sustainable sanitation system based on expanded structured decision-making for global sanitation and resources crisis".JOURNAL OF CLEANER PRODUCTION 21.20(2021):15809-15826. |
入库方式: OAI收割
来源:生态环境研究中心
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