Seasonal dynamics of soil microbial diversity and functions along elevations across the treeline
文献类型:期刊论文
作者 | Shen, Congcong; He, Ji-Zheng; Ge, Yuan |
刊名 | SCIENCE OF THE TOTAL ENVIRONMENT
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出版日期 | 2021-11-15 |
卷号 | 420页码:- |
关键词 | Biochar Oxygenated functional group Water pollution control Adsorption Redox reaction |
ISSN号 | 0304-3894 |
英文摘要 | Biochar has attracted increasing attention in water pollution control, attributed to its various merits, e.g., tunable physico-chemical properties. The oxygenated functional groups (OFGs) on biochar are key active sites for removing pollutants from water through interfacial adsorption/redox reaction. However, there is still a lack of comprehensive knowledge and perspective on tuning OFGs on biochar for enhanced performance in water pollution control. Here, this review highlighted the mechanisms of biochar OFGs in water pollution control, analyzed the strategies and mechanisms for tuning OFGs on biochar, and investigated the performances of biochars with tuned OFGs in removing inorganic/organic pollutants via adsorption/redox reactions. Specifically, strategies for tuning OFGs on biochar are far more than the well-recognized ex-situ oxidation of pristine biochar. These strategies include in-situ low temperature preservation of hydroxyl and carboxyl, in-/ex-situ oxidation of biochar, and in-/ex-situ grafting of carboxyl on biochar via cycloaddition/acylation reaction. The resultant biochars showed enhanced performances in adsorption (mainly mediated by hydroxyl, carboxyl and ketone through surface complexation, H-bonding, and electrostatic attraction) and redox reaction (mainly mediated by redox-active hydroxyl and ketone). Finally, this review presented future directions on developing biochar with specially tuned surface OFGs as a sustainable high-performance adsorbent/carbocatalyst for water pollution control. |
源URL | [https://ir.rcees.ac.cn/handle/311016/46755] ![]() |
专题 | 生态环境研究中心_城市与区域生态国家重点实验室 |
作者单位 | 1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Urban & Reg Ecol, Beijing 100085, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Fujian Normal Univ, Sch Geog Sci, Key Lab Humid Subtrop Ecogeog Proc, Minist Educ, Fuzhou 350007, Peoples R China |
推荐引用方式 GB/T 7714 | Shen, Congcong,He, Ji-Zheng,Ge, Yuan. Seasonal dynamics of soil microbial diversity and functions along elevations across the treeline[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2021,420:-. |
APA | Shen, Congcong,He, Ji-Zheng,&Ge, Yuan.(2021).Seasonal dynamics of soil microbial diversity and functions along elevations across the treeline.SCIENCE OF THE TOTAL ENVIRONMENT,420,-. |
MLA | Shen, Congcong,et al."Seasonal dynamics of soil microbial diversity and functions along elevations across the treeline".SCIENCE OF THE TOTAL ENVIRONMENT 420(2021):-. |
入库方式: OAI收割
来源:生态环境研究中心
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