Distribution, source, and health risk assessment of polycyclic aromatic hydrocarbons in the soils from a typical petroleum refinery area in south China
文献类型：期刊论文
| 作者 | Ma, Wenmin; Hu, Jian ; Li, Jun; Wang, Peng; Okoli, Chukwunonso Peter
|
| 刊名 | ENVIRONMENTAL MONITORING AND ASSESSMENT
 |
| 出版日期 | 2022 |
| 卷号 | 194期号:10页码:678-1-17 |
| 关键词 | Polycyclic aromatic hydrocarbons Principal component analysis Human health risk Petroleum refinery area Soil pollution Carcinogenic risk |
| ISSN号 | 0167-6369 |
| 英文摘要 | The ubiquity of polycyclic aromatic hydrocarbons (PAHs) in soils in petroleum refining areas is an important problem affecting human and ecological safety. In this study, 103 topsoil (0-0.50 m) samples were collected from a retired petroleum refinery area in Guangdong province, south China. The PAHs concentrations were determined by ultrasonic extraction and gas chromatography-mass spectrometry detection methods. Twelve PAHs controlled priority listed by the US Environmental Protection Agency (USEPA) were investigated. The results revealed that the concentration of Sigma(2)PAHs ranged from 2100 to 5200 mg kg(-1), with a mean value of 3741.66 mg kg(-1). The site was dominated by high rings PAHs (4-, 5-, and 6-ring), contributing 81.96% to Sigma(12)PAHs. The concentrations of 9 kinds of PAHs exceeded the Dutch soil quality standard. Besides, the PAHs were primarily distributed in the storage tank area and with high levels of contamination. The results of hierarchical cluster analysis (HCA) and principal component analysis (PCA) indicated that coal combustion was the source of PAHs in topsoil, followed by petroleum dripping and traffic emissions. The incremental lifetime cancer risk (ILCR) modeling illustrated that soil ingestion was the major pathway of PAH exposure for both adults and children. Notably, the total noncarcinogenic human health risk due to PAHs was within the limit of 1, while the carcinogenic risks alone caused by benzo(a)pyrene via soil ingestion to adults and children were obviously beyond the USEPA limit (1.00E-06). Therefore, PAHs in the petroleum refinery areas have potential carcinogenic hazards to human health, the area should be remediated before reuse. |
| 源URL | [https://ir.rcees.ac.cn/handle/311016/48397]  |
| 专题 | 生态环境研究中心_城市与区域生态国家重点实验室 |
| 作者单位 | 1.Chinese Academy of Sciences 2.Tianjin Normal University |
| 推荐引用方式 GB/T 7714 | Ma, Wenmin,Hu, Jian,Li, Jun,et al. Distribution, source, and health risk assessment of polycyclic aromatic hydrocarbons in the soils from a typical petroleum refinery area in south China[J]. ENVIRONMENTAL MONITORING AND ASSESSMENT,2022,194(10):678-1-17. |
| APA | Ma, Wenmin,Hu, Jian,Li, Jun,Wang, Peng,&Okoli, Chukwunonso Peter.(2022).Distribution, source, and health risk assessment of polycyclic aromatic hydrocarbons in the soils from a typical petroleum refinery area in south China.ENVIRONMENTAL MONITORING AND ASSESSMENT,194(10),678-1-17. |
| MLA | Ma, Wenmin,et al."Distribution, source, and health risk assessment of polycyclic aromatic hydrocarbons in the soils from a typical petroleum refinery area in south China".ENVIRONMENTAL MONITORING AND ASSESSMENT 194.10(2022):678-1-17. |
入库方式： OAI收割
来源：生态环境研究中心
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